Hostname: page-component-848d4c4894-2pzkn Total loading time: 0 Render date: 2024-06-03T14:52:52.511Z Has data issue: false hasContentIssue false
  • English
  • Français

Preparation of superhydrophobic and superoleophobic Al–Mg alloy surface via simple, environmentally friendly method

Published online by Cambridge University Press:  10 September 2018

Ning Ma Open the ORCID record for Ning Ma [Opens in a new window] ,
Yang Chen ,
Shuguo Zhao ,
Jingchun Li ,
Baofeng Shan  and
Juhe Sun
Ning Ma*
Affiliation:
School of Mechatronic Engineering, Shenyang Aerospace University, Shenyang 110136, China
Yang Chen
Affiliation:
School of Mechatronic Engineering, Shenyang Aerospace University, Shenyang 110136, China
Shuguo Zhao
Affiliation:
School of Mechatronic Engineering, Shenyang Aerospace University, Shenyang 110136, China
Jingchun Li
Affiliation:
School of Mechatronic Engineering, Shenyang Aerospace University, Shenyang 110136, China
Baofeng Shan
Affiliation:
School of Mechatronic Engineering, Shenyang Aerospace University, Shenyang 110136, China
Juhe Sun
Affiliation:
School of Science, Shenyang Aerospace University, Shenyang 110136, China
*
a)Address all correspondence to this author. e-mail: maning1979@163.com
Get access

Abstract

The micro-nano rough structure promotes the formation of superhydrophobic surfaces, while the formation of superoleophobic surfaces requires the support of re-entrant structures. Electrochemical etching and boiling water treatment methods were used to process the superoleophobic surface in the Al–Mg alloy substrate. The differences between the potential of the aluminum and the magnesium promoted the formation of the surface microstructure under the current stimulation, and the surface was formed into dense nanoscale needle-like coating after boiling water treatment. Scanning electron microscopy, energy dispersive spectroscopy, and contact angle measurement were performed to characterize the morphological features, chemical composition, and surface wettability, respectively. The so-prepared superoleophobic surfaces showed high contact angles and small sliding angles for water, ethylene glycol, and hexadecane. In addition, surface topography, reaction mechanism, and experimental parameters were also studied.

Keywords

alloyenvironmentally benignsurface chemistry
Type
Article
Information
Journal of Materials Research , Volume 33 , Issue 22 , 28 November 2018 , pp. 3818 - 3826
Copyright
Copyright © Materials Research Society 2018 

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

REFERENCES

Liu, K., Tian, Y., and Jiang, L.: Bio-inspired superoleophobic and smart materials: Design, fabrication, and application. Prog. Mater. Sci. 58, 503 (2013).CrossRefGoogle Scholar
Darmanin, T. and Guittard, F.: Superhydrophobic and superoleophobic properties in nature. Mater. Today 18, 273 (2015).CrossRefGoogle Scholar
Lu, Y., Xu, W., Song, J., Liu, X., Xing, Y., and Sun, J.: Preparation of superhydrophobic titanium surfaces via electrochemical etching and fluorosilane modification. Appl. Surf. Sci. 263, 297 (2012).CrossRefGoogle Scholar
Feng, L., Che, Y., Liu, Y., Qiang, X., and Wang, Y.: Fabrication of superhydrophobic aluminium alloy surface with excellent corrosion resistance by a facile and environment-friendly method. Appl. Surf. Sci. 283, 367 (2013).CrossRefGoogle Scholar
Li, X., Zhang, Q., Guo, Z., Shi, T., Yu, J., Tang, M., and Huang, X.: Fabrication of superhydrophobic surface with improved corrosion inhibition on 6061 aluminum alloy substrate. Appl. Surf. Sci. 342, 76 (2015).CrossRefGoogle Scholar
Liang, M., Wei, Y., Hou, L., Wang, H., Li, Y., and Guo, C.: Fabrication of a super-hydrophobic surface on a magnesium alloy by a simple method. J. Alloys Compd. 656, 311 (2016).CrossRefGoogle Scholar
Esmaeilirad, A. and Rukosuyev, M.V.: A cost-effective method to create physically and thermally stable and storable super-hydrophobic aluminum alloy surfaces. Surf. Coat. Technol. 285, 227 (2016).CrossRefGoogle Scholar
Young, T.: An essay on the cohesion of fluids. Philos. Trans. R. Soc. London 95, 65 (1804).CrossRefGoogle Scholar
Tsujii, K., Yamamoto, T., Onda, T., and Shibuichi, S.: Super oil-repellent surfaces. Angew. Chem., Int. Ed. Engl. 36, 9 (1997).CrossRefGoogle Scholar
Tuteja, A., Choi, W., Ma, M., Mabry, J.M., Mazzella, S.A., Rutledge, G.C., McKinley, G.H., and Cohen, R.E.: Designing superoleophobic surfaces. Science 318, 1618 (2007).CrossRefGoogle ScholarPubMed
Song, J., Huang, S., Hu, K., Lu, Y., Liu, X., and Xu, W.: Fabrication of superoleophobic surfaces on Al substrates. J. Mater. Chem. A 1, 14783 (2013).CrossRefGoogle Scholar
Saifaldeen, Z.S., Khedir, K.R., Cansizoglu, M.F., Demirkan, T., and Karabacak, T.: Superamphiphobic aluminum alloy surfaces with micro and nanoscale hierarchical roughness produced by a simple and environmentally friendly technique. J. Mater. Sci. 49, 1839 (2013).CrossRefGoogle Scholar
Cheng, F.J., Yao, J.F., Yang, Z.W., Wang, Y., and Xiao, B.: Structure and composition of oxide film on 5083 alloy at brazing temperature. Mater. Sci. Technol. 31, 1282 (2015).CrossRefGoogle Scholar
Tuan, N.Q., Alves, A.C., Toptan, F., Lopes, A.B., and Pinto, A.M.P.: The effect of Sc and Yb microalloying additions and aged-hardening heat treatment on corrosion behavior of Al–Mg alloys. Mater. Corros. 67, 60 (2016).CrossRefGoogle Scholar
Liu, Y., Liu, J., and Li, S.: One-step method for fabrication of biomimetic superhydrophobic surface on aluminum alloy. Colloids Surf., A 466, 125 (2015).CrossRefGoogle Scholar
Golumbfskie, W., Tran, K.N., and Noland, J.: Survey of detection, mitigation, and repair technologies to address problems caused by sensitization of Al–Mg allows on navy ships. Corrosion 72, 314 (2015).CrossRefGoogle Scholar
Shi, T., Kong, J., and Wang, X.: Preparation of multifunctional Al–Mg alloy surface with hierarchical micro/nanostructures by selective chemical etching processes. Appl. Surf. Sci. 389, 335 (2016).CrossRefGoogle Scholar
Guan, L., Zhou, Y., and Zhang, B.: Influence of aging treatment on the pitting behaviour associated with the dissolution of active nanoscale β-phase precipitates for an Al–Mg alloy. Corros. Sci. 103, 255 (2015).CrossRefGoogle Scholar
Wang, B., Liu, J., and Yin, M.: Comparison of corrosion behavior of Al–Mn and Al–Mg alloys in chloride aqueous solution. Mater. Corros. 67, 51 (2015).CrossRefGoogle Scholar
Peng, S. and Bhushan, B.: Mechanically durable superoleophobic aluminum surfaces with microstep and nanoreticula hierarchical structure for self-cleaning and anti-smudge properties. J. Colloid Interface Sci. 461, 273 (2016).CrossRefGoogle ScholarPubMed
Motlagh, N.V., Birjandi, F.C., Sargolzaei, J., and Shahtahmassebi, N.: Durable, superhydrophobic, superoleophobic and corrosion resistant coating on the stainless steel surface using a scalable method. Appl. Surf. Sci. 283, 636 (2013).CrossRefGoogle Scholar
Al-Milaji, K.N. and Zhao, H.: Fabrication of superoleophobic surfaces by mask-assisted electrospray. Appl. Surf. Sci. 396, 955 (2017).CrossRefGoogle Scholar
Hsieh, C.T. and Wu, F.L.: Superhydrophobicity and superoleophobicity from hierarchical silica sphere stacking layers. Mater. Chem. Phys. 121, 14 (2010).CrossRefGoogle Scholar
Liu, Y., Li, S., and Wang, Y.: Superhydrophobic and superoleophobic surface by electrodeposition on magnesium alloy substrate: Wettability and corrosion inhibition. J. Colloid Interface Sci. 478, 164 (2016).CrossRefGoogle ScholarPubMed
Choi, H.J., Shin, J.H., Choo, S., Ryu, S.W., Kim, Y.D., and Lee, H.: Fabrication of superhydrophobic and oleophobic Al surfaces by chemical etching and surface fluorination. Thin Solid Films 585, 76 (2015).CrossRefGoogle Scholar
Vedder, W. and Vermilyea, D.A.: Aluminum + Water reaction. Trans. Faraday Soc. 65, 561 (1969).CrossRefGoogle Scholar
McCarvill, W.T. and Bell, J.P.: The effect of time and type of water pretreatment on the bond strength of epoxy–aluminum joints. J. Appl. Polym. Sci. 18, 335 (2010).CrossRefGoogle Scholar
Supplementary material: Image

Ma et al. supplementary material

Figure S1

Download Ma et al. supplementary material(Image)
Image 974.4 KB
Supplementary material: Image

Ma et al. supplementary material

Figure S2

Download Ma et al. supplementary material(Image)
Image 974.4 KB
Supplementary material: Image

Ma et al. supplementary material

Figure S3

Download Ma et al. supplementary material(Image)
Image 977.5 KB
Supplementary material: Image

Ma et al. supplementary material

Figure S4

Download Ma et al. supplementary material(Image)
Image 974.4 KB
Supplementary material: Image

Ma et al. supplementary material

Figure S5

Download Ma et al. supplementary material(Image)
Image 989.9 KB