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Nanoprobe Fourier-Transform Photoabsorption Spectroscopy Using a Supercontinuum Light Source

  • Kiyoshiro Ishibe (a1), Satoru Nakada (a1), Yutaka Mera (a1) and Koji Maeda (a1)

A scheme of photoabsorption spectroscopy based on scanning tunneling microscopy (STM) has been developed by using a supercontinuum light as the wideband light source of a Fourier transform interferometer for spectroscopic measurements. The performance was demonstrated for a sample of GaAs. The proof-of-concept test showed that the use of the supercontinuum light instead of halogen lamps greatly enhances the signal-to-noise ratio due to the high brilliance of the supercontinuum light emitted from a small core of the photonic crystal fiber that enables tight focusing of the spectroscopy light onto the sample beneath the STM tip.

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M.S. Anderson (2000). Locally enhanced Raman spectroscopy with an atomic force microscope. Appl Phys Lett 76(21), 31303132.

N. Anderson , A. Hartschuh , S. Cronin & L. Novotny (2005). Nanoscale vibrational analysis of single-walled carbon nanotubes. J Am Chem Soc 127(8), 25332537.

J. Azoulay , A. Deâbarre , A. Richard & P. Tcheânio (1999). Field enhancement and apertureless near-field optical spectroscopy of single molecules. J Microsc 194(2-3), 486490.

S. Berweger , C.C. Neacsu , Y. Mao , H. Zhou , S.S. Wong & M.B. Raschke (2009). Optical nanocrystallography with tip-enhanced phonon Raman spectroscopy. Nat Nanotechnol 4, 496499.

H. Bielefeldt , I. Hörsch , G. Krausch , M. Lux-Steiner , J. Mlynek & O. Marti (1994). Reflection-scanning near-field optical microscopy of opaque samples. Appl Phys A 59(2), 103108.

J.L. Bubendorff , D. Pastreâ & M. Troyon (2000). Cathodoluminescence imaging and spectroscopy by near-field detection. J Microsc 199(3), 191196.

E.S. Carmichael , J.B. Ballard , J.W. Lyding & M. Gruebele (2007). Frequency-modulated, single-molecule absorption detected by scanning tunneling microscopy. J Phys Chem C 111(8), 33143321.

A. Dazzi , R. Prazeres , F. Glotin & J.M. Ortega (2005). Local infrared microspectroscopy with subwavelength spatial resolution with an atomic force microscope tip used as a photothermal sensor. Opt Lett 30 (18), 23882390.

J.M. Dudley , G. Genty & S. Coen (2006). Supercontinuum generation in photonic crystal fiber. Rev Mod Phys 78(4), 11351184.

Ph. Dumas , M. Gu , C. Syrykh , A. Hallimaoui , F. Salvan , J.K. Gimzewski & R.R. Schlittler (1994). Photon spectroscopy, mapping, and topography of 85% porous silicon. J Vac Sci Technol B 12(3), 20642066.

M. Fujihira , H. Monobe , H. Muramatsu & T. Ataka (1994). Scanning near-field microscopy and nanoscopic fluorescence spectroscopy in combination with a non-contact scanning force microscope. Chem Lett 23, 657660.

S. Grafström (2002). Photoassisted scanning tunneling microscopy. J Appl Phys 91(4), 17171753.

A. Hammiche , H.M. Pollock , M. Reading , M. Claybourn , P.H. Turner & K. Jewkes (1999). Photothermal FT-IR spectroscopy: A step towards FT-IR microscopy at a resolution better than the diffraction limit. Appl Spectrosc 53(7), 810815.

N. Hayazawa , Y. Inouye , Z. Sekkat & S. Kawata (2000). Metallized tip amplification of near-field Raman scattering. Opt Comm 183, 333336.

A. Hida , Y. Mera & K. Maeda (2001a). Electric field modulation spectroscopy by scanning tunneling microscopy with a nanometer-scale resolution. Appl Phys Lett 78(20), 30293031.

A. Hida , Y. Mera & K. Maeda (2001b). Nanometer-scale measurements of photoabsorption spectra of individual defects in semiconductors. Appl Phys Lett 78(21), 31903192.

A.J. Huber , A. Ziegler , T. Köck & R. Hillenbrand (2009). Infrared nanoscopy of strained semiconductors. Nat Nanotechnol 4, 153157.

M.S. Jeong , J.Y. Kim , Y.-W. Kim , J.O. White , E.-K. Suh , C.-H. Hong & H.J. Lee (2001). Spatially resolved photoluminescence in InGaN/GaN quantum wells by near-field scanning optical microscopy. Appl Phys Lett 79(7), 976978.

N. Naruse , Y. Mera , Y. Fukuzawa , Y. Nakamura , M. Ichikawa & K. Maeda (2007a). Fourier transform photoabsorption spectroscopy based on scanning tunneling microscopy. J Appl Phys 102(11), 114301-1–6.

N. Naruse , Y. Mera & K. Maeda (2007b). Response analysis for identifying the origin of photo-modulated current contrasts in scanning tunneling microscopic imaging semiconductor surfaces. Ultramicroscopy 107(8), 568574.

N. Naruse , Y. Mera , Y. Nakamura , M. Ichikawa & K. Maeda (2009). Fourier-transform photoabsorption spectroscopy of quantum-confinement effects in individual GeSn nanodots. Appl Phys Lett 94(9), 093104-1–3.

T. Okuda , T. Eguchi , K. Akiyama , A. Harasawa , T. Kinoshita , Y. Hasegawa , M. Kawamori , Y. Haruyama & S. Matsui (2009). Nanoscale chemical imaging by scanning tunneling microscopy assisted by synchrotron radiation. Phys Rev Lett 102(10), 105503-1–4.

B. Pettinger , B. Ren , G. Picardi , R. Schuster & G. Ertl (2004). Nanoscale probing of adsorbed species by tip-enhanced Raman spectroscopy. Phys Rev Lett 92(9), 096101-1–4.

A. Saito , Y. Takagi , K. Takahashi , H. Hosokawa , K. Hanai , T. Tanaka , M. Akai-kasaya , Y. Tanaka , S. Shin , T. Ishikawa , Y. Kuwahara & M. Aono (2008). Nanoscale elemental identification by synchrotron-radiation-based scanning tunneling microscopy. Surf Interf Anal 40(6-7), 10331036.

O. Takeuchi , M. Aoyama , R. Oshima , Y. Okada , H. Oigawa , N. Sano , H. Shigekawa , R. Morita & M. Yamashita (2004). Probing subpicosecond dynamics using pulsed laser combined scanning tunneling microscopy. Appl Phys Lett 85(15), 32683270.

Y. Toda , S. Shinomori , K. Suzuki & Y. Arakawa (1998). Near-field optical spectroscopy of self-assembled quantum dots: NSOM apparatus for measuring the features of single dots. Solid-State Electron 42, 10831086.

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Microscopy and Microanalysis
  • ISSN: 1431-9276
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