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14C and 10Be in Dust Deposited During the Storm of 16–17 April 2006 in Beijing

  • C D Shen (a1), W X Yi (a1), P Ding (a1), K X Liu (a2) and X M Xu (a3)...

Abstract

The concentrations of 10Be and 14C and values of δ13C in samples collected during a major dust storm in Beijing on 16–17 April 2006 were studied. The 10Be concentrations ranged from 1.69 × 108 to 2.07 × 108 atom/g, 14C ages for black carbon (BC) ranged from 3001 to 5181 yr BP and for total inorganic carbon (TIC) from 8464 to 9119 yr BP, and δ13C values for BC ranged from -23.15% to -23.80% and for TIC from -5.39% to -5.98%. A comparison of BC content and δ13C value between the dust, surface soil in the dust source region, and aerosols in Beijing indicated that BC in the dust deposited in Beijing is significantly incorporated by aerosol BC during the dust transportation. Based on the 14C ages of BC, the proportion of fossil-fuel-derived BC was 0.35–0.49 of the total. In contrast to BC, the TIC deposited in Beijing can be firmly related to the source area and δ13C was not significantly modified during its transportation. According to the 14C ages of TIC, the proportion of the secondary carbonate in the dust was from 0.63 to 0.70. The results confirm that 14C of TIC is another useful tracer to indicate the source region of dust besides the content and δ13C value of TIC from the arid and semi-arid regions of China.

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Corresponding author

2 Corresponding author. Email address: cdshen@gig.ac.cn.

References

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Bao, G, Wu, Q, Alatenguya, , Bao, YH. 2012. Changes in temperature and precipitation during past 30 years in Inner Mongolia. Journal of Inner Mongolia Normal University 41(6):668–74. In Chinese with English abstract.
Beer, J, Shen, CD, Heller, F, Liu, TS, Bonani, G, Beate, D, Suter, M, Kubik, PW. 1993. 10Be and magnetic susceptibility in Chinese loess. Geophysical Research Letters 20(1):5760.
Bird, MI, Veenendaal, E, Moyo, C, Veenendaal, EM, Lloyd, J, Frost, P. 1999. Stability of elemental carbon in a savanna soil. Global Biogeochemical Cycles 13(4):923–32.
Bond, TC, Streets, DG, Yarber, KF. 2004. A technology-based global inventory of black and organic carbon emission from combustion. Journal of Geophysical Research Atmospheres 109: D14203, doi:10.1029/2003JD003697.
Cao, JJ, Chow, JC, Tao, J, Lee, SC, Watson, JG, Ho, KF, Wang, GH, Zhu, CS, Han, YM. 2011. Stable carbon isotopes in aerosols from Chinese cities: influence of fossil fuels. Atmospheric Environment 45(6):1359–63.
Cao, JJ, Lee, SC, Zhang, XY, Chow, JC, An, ZS, Ho, KF, Watson, JG, Fung, K, Wang, YQ, Shen, ZX. 2005. Characterization of airborne carbonate over a site near Asian dust source regions during spring 2002 and its climatic and environmental significance. Journal of Geophysical Research 110: D03203, doi:10.1029/2004JD005244.
Cao, JJ, Wang, YQ, Zhang, XY, Lee, SC, Ho, KF, Cao, YN, Li, Y. 2004. Analysis of carbon isotopes in airborne carbonate and implications for aeolian sources. Chinese Science Bulletin 49(15):1637–41.
Cerling, TE. 1984. The stable isotopic composition of modern soil carbonate and its relationship to climate. Earth and Planetary Science Letters 71(2):229–40.
Cerling, TE, Quade, J, Wang, Y, Bowman, JR. 1989. Carbon isotope in soils and palaeosols as ecology and palaeoecology indicators. Nature 341(6238): 138–9.
Chen, B, Kitagawa, H, Jie, DM, Hu, K, Lim, J. 2008. Dust transport from northeastern China inferred from carbon isotopes of atmospheric dust carbonate. Atmospheric Environment 42(19):4790–6.
Chen, QM, Wang, SQ, Yu, G. 2003. Spatial characteristics of soil organic carbon and nitrogen in Inner Mongolia. Chinese Journal of Applied Ecology 14(5):699704.
Chen, S, Liao, S, Jian, W. 1997. Particle size distribution of aerosol carbons in ambient air. Environment International B 23(4):475–88.
Chylek, P, Johnson, B, Wu, H. 1992. Black carbon concentration in a Greenland dye-3 ice core. Geophysical Research Letters 19(19):1951–3.
Currie, LA, Benner, BA, Kessler, JD. 2002. A critical evaluation of inter laboratory data on total elemental, and isotopic carbon in the carbonaceous particle reference material, NIST SRM 1649a. Journal of Research of the National Institute of Standards and Technology 107(3):279–98.
Gu, ZY, Lal, D, Liu, TS. Southon, J, Caffee, MW, Guo, ZT, Chen, MY. 1996. Five million year 10Be record in Chinese loess and red-clay: Climate and weathering relationships. Earth and Planetary Science Letters 144(1–2):273–87.
Gu, ZY, Lal, D, Liu, TS. Guo, ZT, Southon, J, Caffee, MW. 1997. Weathering histories of Chinese loess deposits based on uranium and thorium series nuclides and cosmogenic 10Be. Geochimica et Cosmochimica Acta 61(24):5221–31.
Han, TL, Lin, JX, Wang, Y, Zheng, BY, Song, HL, Liu, JY, Jiang, GM, Shi, PJ, Zhang, J. 2007. Nature and control of dust storms in the Beijing-Tianjin region, China—a case study of the dust storm in Beijing on April 16, 2006. Geological Bulletin of China 26(2):117–27. In Chinese with English abstract.
Heller, F, Shen, CD, Beer, J, Liu, XM, Liu, TS, Bronger, A, Suter, M, Bonani, G. 1993. Quantitative estimates of pedogenic ferromagnetic mineral formation in Chinese loess and palaeoclimatic implications. Earth and Planetary Science Letters 114(2–3):385–90.
Huang, J, Kang, SC, Shen, CD, Cong, ZY, Liu, KX, Wang, W, Liu, LC. 2010. Seasonal variations and sources of ambient fossil and biogenic-derived carbonaceous aerosols based on 14C measurements in Lhasa, Tibet. Atmosphere Research 96(4):553–9.
In, HJ, Park, SU. 2003. The soil particle size dependent emission parameterization for an Asian dust (Yellow Sand) observed in Korea in April 2002. Atmospheric Environment 37(33):4625–36.
Kim, KH, Kim, MY. 2003. The effects of Asian dust on particulate matter fractionation in Seoul, Korea during spring of 2001. Chemosphere 51(8):707–21.
Kwon, HJ, Cho, SH, Chun, Y, Lagarde, F, Pershgen, G. 2002. Effects of the Asian dust events on daily mortality in Seoul, Korea. Environmental Research A 90(1): 15.
Lal, D. 2007. Recycling of cosmogenic nuclides after their removal from the atmosphere; special case of appreciable transport of 10Be to polar regions by aeolian dust. Earth and Planetary Science Letters 264(1–2): 177–87.
Levin, I, Hesshaimer, V. 2000. Radiocarbon—a unique tracer of global carbon cycle dynamics. Radiocarbon 42(1):6980.
Levin, I, Kromer, B, Schmidt, M, Sartorius, H. 2003. A novel approach for independent budgeting of fossil fuel CO2 over Europe by 14CO2 observations. Geophysical Research Letters 30(23):2194, doi:10.1029/2003GL018477.
Lim, B, Cachier, H. 1996. Determination of black carbon by chemical oxidation and thermal treatment in recent marine and lake sediments and Cretaceous-Tertiary clays. Chemical Geology 131(1–4):143–54.
Lim, JY, Chun, Y. 2006. The characteristics of Asian dust events in northeast Asia during the springtime from 1993 to 2004. Global and Planetary Change 52(1–4): 231–47.
Liu, K, Ding, X, Fu, D, Pan, Y, Wu, X, Guo, Z, Zhou, L. 2007. A new compact AMS system at Peking University. Nuclear Instruments and Methods in Physics Research B 259(1):23–6.
Liu, T, Ding, Z. 1998. Chinese loess and the paleomonsoon. Annual Review of Earth and Planetary Science 26:111–45
Liu, T, Han, JM, Zhang, D, Qin, XG, Zhang, S, Jin, CS, Liu, P, Jiang, WL. 2006. Falling dust and deposition in anthropogene I:preliminary analyses of the dust in Beijing on April 16–17, 2006. Quaternary Sciences 26(4):628–33. In Chinese with English abstract.
, YW, Gu, ZY, Aldanhan, Ala, Zhang, HC, Possnert, G, Lei, GL. 2010. 10Be in quartz gravel from the Gobi Desert and evolutionary history of alluvial sedimentation in the Ejina Basin, Inner Mongolia, China. Chinese Science Bulletin 55(33):3802–9
Ning, YF, Liu, WG, An, ZS. 2006. Variation of soil δΔ13C values in Xifeng loess-paleosol sequence and its paleoenvironmental implication. Chinese Science Bulletin 51(11):1350–4.
Shen, CD. 1986. Beryllium-10 in Chinese loess [PhD thesis]. Universtät Bern.
Shen, CD, Beer, J, Liu, T S, Oeschger, H, Bonani, G, Suter, M, Wölfli, W. 1992. 10Be in Chinese loess. Earth and Planetary Science Letters 109 (1–2):169–77.
Shen, CD, Ding, P, Wang, N, Han, J, Zhang, S, Liu, K, Ding, X, Fu, D. 2007. Distribution of cosmogenic 14C and 10Be of fall dust in Beijing on April 16–17, 2006. Quaternary Sciences 27(6):919–33. In Chinese with English abstract.
Shen, CD, Liu, TS, Beer, J, Oeschger, H, Bonani, G, Suter, M, Wolfli, W. 1987. 10Be in Chinese loess. In: Liu, TS, editor. Aspects of Loess Research. Beijing: China Ocean Press. p 277–82.
Shen, CD, Yi, WX, Sun, YM, Xing, CP, Yang, Y, Yuan, C, Li, Z, Peng, SL, An, ZS, Liu, TS. 2001. Distribution of 14C and 13C in forest soils of Dinghushan Biosphere Reserve. Radiocarbon 43(2B):671–8.
Smith, DM, Griffin, JJ, Goldberg, ED. 1975. Spectrometric method for quantitative-determination of elemental carbon. Analytical Chemistry 47(2):233–8.
Suter, M, Balzer, R, Bonani, G, Hofmann, H, Morenzoni, E, Nessi, M, Wölfli, W. 1984. Precision measurements of 14C in AMS-some results and prospects. Nuclear Instruments and Methods in Physics Research B 5(2): 117–22.
Tang, Y, Han, GL, Xu, ZF. 2013. Black carbon in the atmospheric dust of Beijing City and its north area. Acta Scientiae Circumstantiae 33(2):332–8. In Chinese with English abstract.
Uematsn, M, Wang, ZF, Uno, I. 2003. Atmospheric input of mineral dust to the western North Pacific region based on direct measurements and a regional chemical transport model. Geophysical Research Letters 30(6): 1342.
Wang, YQ, Cao, JJ, Zhang, XY, Shen, ZX, Mei, ZX. 2004. Carbonate content and carbon and oxygen isotopic composition of surface soil in the dust source regions of China. Marine Geology & Quaternary Geology 24(1):113–17. In Chinese with English abstract.
Wang, YQ, Zhang, XY, Arimoto, R, Cao, JJ, Shen, ZX. 2005. Characteristics of carbonate content and carbon and oxygen isotopic composition of northern China soil and dust aerosol and its application to tracing dust sources. Atmospheric Environment 39(14):2631–42.
Wen, QZ. 1989. Geochemical Research on Chinese Loess. Beijing: Science Press. p 115–44. In Chinese.
Xu, XM, Trumbore, SE, Zheng, SH, Southon, JR, McDuffee, KE, Luttgen, M, Liu, JC. 2007. Modifying a sealed tube zinc reduction method for preparation of AMS graphite targets: reducing background and attaining high precision. Nuclear Instruments and Methods in Physics Research B 259(1):320–9.
Zhang, S, Heller, F, Jin, CS, Liu, P, Qin, XG, Liu, TS. 2008. Grain size distribution and magnetic characteristics of dust fall in Beijing on April 17, 2006. Quaternary Sciences 28(2):354–62.
Yang, F He, K, Chen, X, Cha, L, Cadle, SH, Chan, T, Mulawa, PA. 2005. One-year record of organic and elemental carbon in fine particles in downtown Beijing and Shanghai. Atmospheric Chemistry and Physics 5: 1449–57.
Yang, Y, Shen, CD, Yi, WX, Sun, YM, Liu, TS. 2001. The elemental carbon record in Weinan loess section since the last 21ka. Chinese Science Bulletin 46(18):1541–4.
Zhang, S, Heller, F, Jin, CS, Liu, P, Qin, XG, Liu, TS. 2008. Grain size distribution and magnetic characteristics of dust fall in Beijing on April 17, 2006. Quaternary Sciences 28(2):354–62. In Chinese with English abstract.
Zhang, T, Dong, XH. 2002. Carbonate carbon measurement in sand storm and dust storm source identification. Environmental monitoring in China 18(2):11–4.
Zhang, XY, Arimoto, R, An, ZS. 1997. Dust emission from Chinese desert sources linked to variations in atmospheric circulation. Journal of Geophysical Research 102(D23):28,04147.
Zhou, B, Shen, CD, Sun, WD, Yang, Y, Sun, YB, An, ZS. 2007. Elemental carbon record of paleofire history on the Chinese Loess Plateau during the last 420 ka and its response to environmental and climate changes. Palaeogeography, Palaeoclimatology, Palaeoecology 252(3–4):617–25.

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