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Direct Observation of Electrolyte Degradation Mechanisms in Li-Ion Batteries

Published online by Cambridge University Press:  27 August 2014

B. Layla Mehdi ,
Patricia Abellan ,
Lucas R. Parent ,
Meng Gu ,
Chiwoo Park ,
Wu Xu ,
Yaohui Zhang ,
Ilke Arslan ,
Ji-Guang Zhang  and
Chong-Min Wang
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B. Layla Mehdi
Affiliation:
.Fundamental and Computational Sciences Directorate, Pacific Northwest National Laboratory, Richland, WA, USA
Patricia Abellan
Affiliation:
.Fundamental and Computational Sciences Directorate, Pacific Northwest National Laboratory, Richland, WA, USA
Lucas R. Parent
Affiliation:
.Fundamental and Computational Sciences Directorate, Pacific Northwest National Laboratory, Richland, WA, USA
Meng Gu
Affiliation:
.Environmental Molecular Science Laboratory, Pacific Northwest National Laboratory, Richland, WA, USA
Chiwoo Park
Affiliation:
.Department of Industrial and Manufacturing Engineering, Florida State University, Tallahassee, FL,USA
Wu Xu
Affiliation:
.Energy and Environmental Directorate, Pacific Northwest National Laboratory, Richland, WA, USA
Yaohui Zhang
Affiliation:
.Energy and Environmental Directorate, Pacific Northwest National Laboratory, Richland, WA, USA .Center for Condensed Matter Science and Technology, Department of Physics, Harbin Institute of Technology, PR China
Ilke Arslan
Affiliation:
.Energy and Environmental Directorate, Pacific Northwest National Laboratory, Richland, WA, USA
Ji-Guang Zhang
Affiliation:
.Energy and Environmental Directorate, Pacific Northwest National Laboratory, Richland, WA, USA
Chong-Min Wang
Affiliation:
.Environmental Molecular Science Laboratory, Pacific Northwest National Laboratory, Richland, WA, USA
James E. Evans
Affiliation:
.Environmental Molecular Science Laboratory, Pacific Northwest National Laboratory, Richland, WA, USA
Nigel D. Browning
Affiliation:
.Fundamental and Computational Sciences Directorate, Pacific Northwest National Laboratory, Richland, WA, USA

Abstract

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Abstract
Information
Microscopy and Microanalysis , Volume 20 , Supplement S3: Proceedings of Microscopy & Microanalysis 2014 , August 2014 , pp. 1624 - 1625
Copyright
Copyright © Microscopy Society of America 2014 

References

[1] Xu, K., Chem, K. Rev., 104 (2004), p. 4303.Google Scholar
[2] Nasybulin, E., Xu, W., Engelhard, M. H., Nie, Z. M., Burton, S. D., Cosimbescu, L., Gross, M. E., Zhang, J. G. J Phys Chem C, 117 (2013), p. 2635.Google Scholar
[3] Verma, P., Maire, P., Novak, P. Electrochim Acta 55 (2010), p. 6332.Google Scholar
[4] The research described in this paper is part of the Chemical Imaging Initiative; it was conducted under the Laboratory Directed Research and Development Program at PNNL, a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. The electrolytes used in this work were prepared with the support from Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. Development of in-situ stages was supported by DOE NNSA-SSAA grant number DE-FG52-06NA26213, and DOE BES grant number DE-FG02-03ER46057. C.P. acknowledges support from the FSU COFRS Award 032968, the Ralph E. Powe Junior Faculty Enhancement Award, and NSF-CMMI-1334012.Google Scholar