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A Study of Radiation Effects in Curium-Doped Gd2Ti2O7 (Pyrochlore) and CaZrTi2O7 (Zirconolite)*

Published online by Cambridge University Press:  15 February 2011

J.W. Wald
Affiliation:
Pacfic Northwest Laboratory, P.O. Box 999, Richland, Washington, 99352, USA.
P. Offemann
Affiliation:
Hahn-Meitner-Institut fűr Kernforschung Berlin, Glienicker Strasse 100, Postfach 39 01 28, D1000 Berlin 39, Germany.
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Extract

Radiation effects studies in both glass and glass ceramic nuclear waste forms have identified a rare-earth titanate phase of the general formula (RE) 2Ti207 which is capable of acting as a host phase for actinides.1,2 Ringwood and co-workers3 have also proposed a structurally similar phase, zirconolite (CaZrTi2 07), as one of the primary host phases in the SYNROC waste form. Data from these and other previous studies, as well as mineralogical information available on these titanate phases, have not provided an unambiguous interpretation of the effects of radiation damage relative to nuclear waste forms. This paper reports new laboratory data concerning radiation damage effects in both of these phases.

Type
Research Article
Copyright
Copyright © Materials Research Society 1982

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Footnotes

*

This work was supported by the U.S. Department of Energy under contract DE-AC06-76RLO 1830.

References

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