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Catalytic Fe-Oxo Clusters Stabilized on the MOF-808 Metal Organicframework for the Degradation of Water Pollutants

11 September 2020, Version 1
Working Paper
This content is an early or alternative research output and has not been peer-reviewed by Cambridge University Press at the time of posting.

Abstract

Stabilizing catalytic iron-oxo-clusters within nanoporous metal-organic frameworks (MOF) is a powerful strategy to prepare new active materials for the degradation of toxic chemicals, such as bisphenol A. Herein, we combine pair distribution function analysis of total X-ray scattering data and X-ray absorption spectroscopy, with computational modelling to understand the local structural nature of added redox-active iron-oxo clusters bridging neighbouring zirconia-nodes within MOF-808.

Keywords

metal-organic frameworks (MOFs)
Pair Distribution Function Analysis
Pollutants Removal

Supplementary materials

Title
Description
Actions
Title
Fe-MOF-808 ESI Platero-Prats
Description
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Now Published

Unravelling the local structure of catalytic Fe-oxo clusters stabilized on the MOF-808 metal organic-framework [opens in a new tab]
Celia Castillo-Blas, Ignacio Romero-Muñiz, Andreas Mavrandonakis, Laura Simonelli, Ana E. Platero-Prats journal article
Chemical Communications , Volume 56, Issue 100
Online publication date: 2020

Version History

Sep 11, 2020 Version 1

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The content is available under CC BY NC ND 4.0 [opens in a new tab]

DOI

10.26434/chemrxiv.12937691.v1
D O I: 10.26434/chemrxiv.12937691.v1 [opens in a new tab]

Funding

RTI2018-096138-A-I00
2017-T1/IND5148
CALIPSOplus (Grant Agreement 730872 from the EU Framework Programme for Research and Innovation HORIZON 2020).
PEJD-2018-POST/IND-7909
RTI2018-101049-BI00
2017-T1/AMB-5264

Author’s competing interest statement

No conflict of interest.

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