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Designing defect spins for wafer-scale quantum technologies

  • William F. Koehl (a1), Hosung Seo (a2), Giulia Galli (a3) and David D. Awschalom (a4)
Abstract
Abstract

The past decade has seen remarkable progress in the development of the nitrogen-vacancy (NV) defect center in diamond, which is one of the leading candidates for quantum information technologies. The success of the NV center as a solid-state qubit has stimulated an active search for similar defect spins in other technologically important and mature semiconductors, such as silicon carbide. If successfully combined with the advanced microfabrication techniques available to such materials, coherent quantum control of defect spins could potentially lead to semiconductor-based, wafer-scale quantum technologies that make use of exotic quantum mechanical phenomena like entanglement. In this article, we describe the robust spin property of the NV center and the current status of NV center research for quantum information technologies. We then outline first-principles computational modeling techniques based on density functional theory to efficiently search for potential spin defects in nondiamond hosts suitable for quantum information applications. The combination of computational modeling and experimentation has proven invaluable in this area, and we describe the successful interplay between theory and experiment achieved with the divacancy spin qubit in silicon carbide.

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J.P. Dowling , G.J. Milburn , Philos. Trans. R. Soc. London Ser. A 361, 1655 (2003).

J.R. Weber , W.F. Koehl , J.B. Varley , A. Janotti , B.B. Buckley , C.G. Van de Walle , D.D. Awschalom , Proc. Natl. Acad. Sci. U.S.A. 107, 8513 (2010).

M.H. Devoret , J.M. Martinis , Quantum Inf. Process. 3, 163 (2004).

D.G. Cory , R. Laflamme , E. Knill , L. Viola , T.F. Havel , N. Boulant , G. Boutis , E. Fortunato , S. Lloyd , R. Martinez , C. Negrevergne , M. Pravia , Y. Sharf , G. Teklemariam , Y.S. Weinstein , W.H. Zurek , Fortschr. Phys. 48, 875 (2000).

C. Monroe , Nature 416, 238 (2002).

C. Monroe , J. Kim , Science 339, 1164 (2013).

R. Hanson , D.D. Awschalom , Nature 453, 1043 (2008).

S. Bertaina , S. Gambarelli , A. Tkachuk , I.N. Kurkin , B. Malkin , A. Stepanov , B. Barbara , Nat. Nanotechnol. 2, 39 (2007).

F. Jelezko , T. Gaebel , I. Popa , A. Gruber , J. Wrachtrup , Phys. Rev. Lett. 92, 076401 (2004).

G. Balasubramanian , P. Neumann , D. Twitchen , M. Markham , R. Kolesov , N. Mizuochi , J. Isoya , J. Achard , J. Beck , J. Tissler , V. Jacques , P.R. Hemmer , F. Jelezko , J. Wrachtrup , Nat. Mater. 8, 383 (2009).

G. Davies , M.F. Hamer , Proc. R. Soc. Lond. A 348, 285 (1976).

A. Lenef , S.C. Rand , Phys. Rev. B Condens. Matter 53, 13441 (1996).

A. Gruber , A. Dräbenstedt , C. Tietz , L. Fleury , J. Wrachtrup , C. von Borczyskowski , Science 276, 2012 (1997).

R.J. Epstein , F.M. Mendoza , Y.K. Kato , D.D. Awschalom , Nat. Phys. 1, 94 (2005).

N.B. Manson , J.P. Harrison , M.J. Sellars , Phys. Rev. B Condens. Matter 74, 104303 (2006).

G.D. Fuchs , V.V. Dobrovitski , R. Hanson , A. Batra , C.D. Weis , T. Schenkel , D.D. Awschalom , Phys. Rev. Lett. 101, 117601 (2008).

A. Batalov , V. Jacques , F. Kaiser , P. Siyushev , P. Neumann , L.J. Rogers , R.L. McMurtrie , N.B. Manson , F. Jelezko , J. Wrachtrup , Phys. Rev. Lett. 102, 195506 (2009).

G.D. Fuchs , V.V. Dobrovitski , D.M. Toyli , F.J. Heremans , C.D. Weis , T. Schenkel , D.D. Awschalom , Nat. Phys. 6, 668 (2010).

M.W. Doherty , N.B. Manson , P. Delaney , L.C.L. Hollenberg , New J. Phys. 13, 025019 (2011).

J.R. Maze , A. Gali , E. Togan , Y. Chu , A. Trifonov , E. Kaxiras , M.D. Lukin , New J. Phys. 13, 025025 (2011).

G.D. Fuchs , A.L. Falk , V.V. Dobrovitski , D.D. Awschalom , Phys. Rev. Lett. 108, 157602 (2012).

F. Jelezko , T. Gaebel , I. Popa , M. Domhan , A. Gruber , J. Wrachtrup , Phys. Rev. Lett. 93, 130501 (2004).

M.V. Gurudev Dutt , L. Childress , L. Jiang , E. Togan , J. Maze , F. Jelezko , A.S. Zibrov , P.R. Hemmer , M.D. Lukin , Science 316, 1312 (2007).

P. Neumann , J. Beck , M. Steiner , F. Rempp , H. Fedder , P.R. Hemmer , J. Wrachtrup , F. Jelezko , Science 329, 542 (2010).

L. Robledo , L. Childress , H. Bernien , B. Hensen , P.F.A. Alkemade , R. Hanson , Nature 477, 574 (2011).

G. de Lange , Z.H. Wang , D. Ristè , V.V. Dobrovitski , R. Hanson , Science 330, 60 (2010).

C.A. Ryan , J.S. Hodges , D.G. Cory , Phys. Rev. Lett. 105, 200402 (2010).

B. Naydenov , F. Dolde , L.T. Hall , C. Shin , H. Fedder , L.C.L. Hollenberg , F. Jelezko , J. Wrachtrup , Phys. Rev. B Condens. Matter 83, 081201(R) (2011).

T. van der Sar , Z.H. Wang , M.S. Blok , H. Bernien , T.H. Taminiau , D.M. Toyli , D.A. Lidar , D.D. Awschalom , R. Hanson , V.V. Dobrovitski , Nature 484, 82 (2012).

G.D. Fuchs , G. Burkard , P.V. Klimov , D.D. Awschalom , Nat. Phys. 7, 789 (2011).

P.C. Maurer , G. Kucsko , C. Latta , L. Jiang , N.Y. Yao , S.D. Bennett , F. Pastawski , D. Hunger , N. Chisholm , M. Markham , D.J. Twitchen , J.I. Cirac , M.D. Lukin , Science 336, 1283 (2012).

E. Togan , Y. Chu , A.S. Trifonov , L. Jiang , J. Maze , L. Childress , M.V.G. Dutt , A.S. Sørensen , P.R. Hemmer , A.S. Zibrov , M.D. Lukin , Nature 466, 730 (2010).

B.B. Buckley , G.D. Fuchs , L.C. Bassett , D.D. Awschalom , Science 330, 1212 (2010).

C.G. Yale , B.B. Buckley , D.J. Christle , G. Burkard , F.J. Heremans , L.C. Bassett , D.D. Awschalom , Proc. Natl. Acad. Sci. U.S.A. 110, 7595 (2013).

D.A. Golter , H. Wang , Phys. Rev. Lett. 112, 116403 (2014).

L.C. Bassett , F.J. Heremans , D.J. Christle , C.G. Yale , G. Burkard , B.B. Buckley , D.D. Awschalom , Science 345, 1333 (2014).

G. Waldherr , Y. Wang , S. Zaiser , M. Jamali , T. Schulte-Herbrüggen , H. Abe , T. Ohshima , J. Isoya , J.F. Du , P. Neumann , J. Wrachtrup , Nature, published online January 29, 2014, http://dx.doi.org/10.1038/nature12919.

W. Pfaff , T.H. Taminiau , L. Robledo , H. Bernien , M. Markham , D.J. Twitchen , R. Hanson , Nat. Phys. 9, 29 (2013).

F. Dolde , I. Jakobi , B. Naydenov , N. Zhao , S. Pezzagna , C. Trautmann , J. Meijer , P. Neumann , F. Jelezko , J. Wrachtrup , Nat. Phys. 9, 139 (2013).

H. Bernien , B. Hensen , W. Pfaff , G. Koolstra , M.S. Blok , L. Robledo , T.H. Taminiau , M. Markham , D.J. Twitchen , L. Childress , R. Hanson , Nature 497, 86 (2013).

W. Pfaff , B.J. Hensen , H. Bernien , S.B. van Dam , M.S. Blok , T.H. Taminiau , M.J. Tiggelman , R.N. Schouten , M. Markham , D.J. Twitchen , R. Hanson , Science 345, 532 (2014).

J.R. Maze , P.L. Stanwix , J.S. Hodges , S. Hong , J.M. Taylor , P. Cappellaro , L. Jiang , M.V. Gurudev Dutt , E. Togan , A.S. Zibrov , A. Yacoby , R.L. Walsworth , M.D. Lukin , Nature 455, 644 (2008).

G. Balasubramanian , I.Y. Chan , R. Kolesov , M. Al-Hmoud , J. Tisler , C. Shin , C. Kim , A. Wojcik , P.R. Hemmer , A. Krueger , T. Hanke , A. Leitenstorfer , R. Bratschitsch , F. Jelezko , J. Wrachtrup , Nature 455, 648 (2008).

B.J. Maertz , A.P. Wijnheijmer , G.D. Fuchs , M.E. Nowakowski , D.D. Awschalom , Appl. Phys. Lett. 96, 092504 (2010).

F. Dolde , H. Fedder , M.W. Doherty , T. Nöbauer , F. Rempp , G. Balasubramanian , T. Wolf , F. Reinhard , L.C.L. Hollenberg , F. Jelezko , J. Wrachtrup , Nat. Phys. 7, 459 (2011).

D.M. Toyli , C.F. de las Casas , D.J. Christle , V.V. Dobrovitski , D.D. Awschalom , Proc. Natl. Acad. Sci. U.S.A. 110, 8417 (2013).

P. Neumann , I. Jakobi , F. Dolde , C. Burk , R. Reuter , G. Waldherr , J. Honert , T. Wolf , A. Brunner , J.H. Shim , D. Suter , H. Sumiya , J. Isoya , J. Wrachtrup , Nano Lett. 13, 2738 (2013).

L.P. McGuinness , Y. Yan , A. Stacey , D.A. Simpson , L.T. Hall , D. Maclaurin , S. Prawer , P. Mulvaney , J. Wrachtrup , F. Caruso , R.E. Scholten , L.C.L. Hollenberg , Nat. Nanotechnol. 6, 358 (2011).

G. Kucsko , P.C. Maurer , N.Y. Yao , M. Kubo , H.J. Noh , P.K. Lo , H. Park , M.D. Lukin , Nature 500, 54 (2013).

L.T. Hall , G.C.G. Beart , E.A. Thomas , D.A. Simpson , L.P. McGuinness , J.H. Cole , J.H. Manton , R.E. Scholten , F. Jelezko , J. Wrachtrup , S. Petrou , L.C.L. Hollenberg , Sci. Rep. 2, 401 (2012).

H.J. Mamin , M. Kim , M.H. Sherwood , C.T. Rettner , K. Ohno , D.D. Awschalom , D. Rugar , Science 339, 557 (2013).

T. Staudacher , F. Shi , S. Pezzagna , J. Meijer , J. Du , C.A. Meriles , F. Reinhard , J. Wrachtrup , Science 339, 561 (2013).

D.M. Toyli , C.D. Weis , G.D. Fuchs , T. Schenkel , D.D. Awschalom , Nano Lett. 10, 3168 (2010).

L.C. Bassett , F.J. Heremans , C.G. Yale , B.B. Buckley , D.D. Awschalom , Phys. Rev. Lett. 107, 266403 (2011).

H. Kato , M. Wolfer , C. Schreyvoge , M. Kunzer , W. Müller-Sebert , H. Obloh , S. Yamasaki , C. Nebel , Appl. Phys. Lett. 102, 151101 (2013).

A. Faraon , C. Santori , Z. Huang , V.M. Acosta , R.G. Beausoleil , Phys. Rev. Lett. 109, 033604 (2012).

J.C. Lee , D.O. Bracher , S. Cui , K. Ohno , C.A. McLellan , X. Zhang , P. Andrich , B. Alemán , K.J. Russell , A.P. Magyar , I. Aharonovich , A.C. Bleszynski Jayich , D.D. Awschalom , E.L. Hu , Appl. Phys. Lett. 105, 261101 (2014).

N. Thomas , R.J. Barbour , Y. Song , M.L. Lee , K.-M.C. Fu , Opt. Express 22, 13555 (2014).

E.R. MacQuarrie , T.A. Gosavi , N.R. Jungwirth , S.A. Bhave , G.D. Fuchs , Phys. Rev. Lett. 111, 227602 (2013).

J. Teissier , A. Barfuss , P. Appel , E. Neu , P. Maletinsky , Phys. Rev. Lett. 113, 020503 (2014).

P. Ovartchaiyapong , K.W. Lee , B.A. Myers , A.C. Bleszynski Jayich , Nat. Commun. 5, 4429 (2014).

H. Seo , A.A. Demkov , Phys. Rev. B: Condens. Matter 84, 045440 (2011).

T. Ogitsu , E. Schwegler , G. Galli , Chem. Rev. 113, 3425 (2013).

A. Zywietz , J. Furthmüller , F. Bechstedt , Phys. Rev. B: Condens. Matter 59, 15166 (1999).

A. Gali , M. Fyta , E. Kaxiras , Phys. Rev. B: Condens. Matter 77, 155206 (2008).

C. Freysoldt , B. Grabowski , T. Hickel , J. Neugebauer , G. Kresse , A. Janotti , C.G. Van de Walle , Rev. Mod. Phys. 86, 253 (2014).

W. Kohn , L.J. Sham , Phys. Rev. 140, A1133 (1965).

A.D. Becke , J. Chem. Phys. 140, 18A301 (2014).

D.M. Ceperley , B.J. Alder , Phys. Rev. Lett. 45, 566 (1980).

J.P. Perdew , A. Zunger , Phys. Rev. B 23, 5048 (1981).

J.P. Perdew , K. Burke , M. Ernzerhof , Phys. Rev. Lett. 77, 3865 (1997).

H. Seo , A.B. Posadas , A.A. Demkov , Phys. Rev. B Condens. Matter 86, 014430 (2012).

C.G. Van de Walle , J. Neugebauer , Appl. Phys. Rev. 95, 3851 (2004).

J.R. Chelikowsky , in Comprehensive Semiconductor Science and Technology, P. Bhattacharya , R. Fornari , H. Kamimura , Eds. (Elsevier, Amsterdam, 2011), vol. 1, pp. 141.

J.P. Perdew , M. Levy , Phys. Rev. Lett. 51, 1884 (1983).

J.H. Skone , M. Govoni , G. Galli , Phys. Rev. B: Condens. Matter 89, 195112 (2014).

C.D. Clark , P.J. Dean , P.V. Harris , Proc. R. Soc. London, Ser. A 277, 312 (1964).

L. Hedin , Phys. Rev. 139, A796 (1965).

M.S. Hybertsen , S.G. Louie , Phys. Rev. Lett. 55, 1418 (1985).

H.-V. Nguyen , T.A. Pham , D. Rocca , G. Galli , Phys. Rev. B Condens. Matter 85, 081101 (2012).

T.A. Pham , H.-V. Nguyen , D. Rocca , G. Galli , Phys. Rev. B Condens. Matter 87, 155148 (2013).

M. Govoni , G. Galli , J. Chem. Theory Comput. 11, 2680 (2015).

A. Alkauskas , J.L. Lyons , D. Steiauf , C.G. Van de Walle , Phys. Rev. Lett. 109, 267401 (2012).

A. Gali , E. Janzén , P. Deák , G. Kresse , E. Kaxiras , Phys. Rev. Lett. 103, 186404 (2009).

W. Chen , A. Pasquarello , J. Phys. Condens. Matter 27, 133202 (2015).

S. Choi , M. Jain , S.G. Louie , Phys. Rev. B Condens. Matter 86, 041202R (2012).

I.B. Bersuker , The Jahn–Teller Effect (Cambridge University Press, Cambridge, UK, 2006).

H. Seo , A.B. Posadas , A.A. Demkov , Phys. Rev. B Condens. Matter 86, 014430 (2012).

J. Buckeridge , C.R.A. Catlow , D.O. Scanlon , T.W. Keal , P. Sherwood , M. Miskufova , A. Walsh , S.M. Woodley , A.A. Sokol , Phys. Rev. Lett. 114, 016405 (2015).

R. Ishikawa , R. Mishra , A.R. Lupini , S.D. Findlay , T. Taniguchi , S.T. Pantelides , S.J. Pennycook , Phys. Rev. Lett. 113, 155501 (2014).

A. Gali , Phys. Status Solidi B 248, 1337 (2011).

P.G. Baranov , I.V. Il’in , E.N. Mokhov , M.V. Muzafarova , S.B. Orlinskii , J. Schmidt , JETP Lett. 82, 441 (2005).

N.T. Son , P. Carlsson , J. Ul Hassan , E. Janzén , T. Umeda , J. Isoya , A. Gali , M. Bockstedte , N. Morishita , T. Ohshima , H. Itoh , Phys. Rev. Lett. 96, 055501 (2006).

N. Mizuochi , S. Yamasaki , H. Takizawa , N. Morishita , T. Ohshima , H. Itoh , J. Isoya , Phys. Rev. B Condens. Matter 66, 235202 (2002).

N.T. Son , Z. Zolnai , E. Janzén , Phys. Rev. B Condens. Matter 68, 205211 (2003).

P.G. Baranov , A.P. Bundakova , A.A. Soltamov , Phys. Rev. B Condens. Matter 83, 125203 (2011).

S.B. Orlinski , J. Schmidt , E.N. Mokhov , P.G. Baranov , Phys. Rev. B Condens. Matter 67, 125207 (2003).

W.E. Carlos , N.Y. Graces , E.R. Glaser , M.A. Fanton , Phys. Rev. B Condens. Matter 74, 235201 (2006).

W.F. Koehl , B.B. Buckley , F.J. Heremans , G. Calusine , D.D. Awschalom , Nature 479, 84 (2011).

V.A. Soltamov , A.A. Soltamova , P.G. Baranov , I.I. Proskuryakov . Phys. Rev. Lett. 108, 226402 (2012).

G. Calusine , A. Politi , D.D. Awschalom , Appl. Phys. Lett. 105, 011123 (2014).

M. Radulaski , T.M. Babinec , K. Müller , K.G. Lagoudakis , J.L. Zhang , S. Buckley , Y.A. Kelaita , K. Alassaad , G. Ferro , J. Vučković , ACS Photonics 2, 14 (2015).

J.Y. Lee , X. Lu , Q. Lin , Appl. Phys. Lett. 106, 041106 (2015).

A.L. Falk , B.B. Buckley , G. Calusine , W.F. Koehl , V.V. Dobrovitski , A. Politi , C.A. Zorman , P.X.-L. Feng , D.D. Awschalom , Nat. Commun. 4, 1819 (2013).

P.V. Klimov , A.L. Falk , B.B. Buckley , D.D. Awschalom , Phys. Rev. Lett. 112, 087601 (2014).

A.L. Falk , P.V. Klimov , B.B. Buckley , V. Ivady , I. Abrikosov , G. Calusine , W.F. Koehl , A. Gali , D.D. Awschalom , Phys. Rev. Lett. 112, 187601 (2014).

A.L. Falk , P.V. Klimov , V. Ivády , K. Szász , D.J. Christle , W.F. Koehl , A. Gali , D.D. Awschalom , Phys. Rev. Lett. 114, 247603 (2015).

D.J. Christle , A.L. Falk , P. Andrich , P.V. Klimov , J. Ul Hassan , N.T. Son , E. Janzén , T. Ohshima , D.D. Awschalom , Nat. Mater. 14, 160 (2015).

M. Widmann , S.-Y. Lee , T. Rendler , N.T. Son , H. Fedder , S. Paik , L.-P. Yang , N. Zhao , S. Yang , I. Booker , A. Denisenko , M. Jamali , S.A. Momenzadeh , I. Gerhardt , T. Ohshima , A. Gali , E. Janzén , J. Wrachtrup , Nat. Mater. 14, 164 (2015).

W.D. Rice , P. Ambwani , M. Bombeck , J.D. Thompson , G. Haugstad , C. Leighton , S.A. Crooker , Nat. Mater. 13, 481 (2014).

N.R. Jungwirth , Y.Y. Pai , H.S. Chang , E.R. MacQuarrie , K.X. Nguyen , G.D. Fuchs , J. Appl. Phys. 116, 043509 (2014).

O.V. Zwier , D. O’Shea , A.R. Onur , C.H. van der Wal , Sci. Rep. 5, 10931 (2015).

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