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Plasmonic excitation and manipulation with an electron beam

  • Ernst Jan R. Vesseur (a1), Javier Aizpurua (a2), Toon Coenen (a3), Alejandro Reyes-Coronado (a4), Philip E. Batson (a5) and Albert Polman (a6)...

When an electron beam passes through or near a metal structure, it will excite surface plasmons, providing a unique way to access surface plasmon behavior at the nanoscale. An electron beam focused to nanometer dimensions thus functions as a point source that is able to probe the local plasmonic mode structure at deep-subwavelength resolution. In this article, we show how well-controlled coupling between an electron beam and surface plasmons, combined with a far-field detection system, allows characterization and manipulation of plasmons on a variety of plasmonic devices. By mapping the spatial profile of inelastic scattering to resonant modes, the dispersion and losses of surface plasmons are resolved. The technique further allows probing of the confinement of plasmons within cavities and measuring the angular emission profile of nanoantennas. The coupling of electrons to surface plasmons allows the use of the electron beam as a dipole emitter that can be positioned at will. The beam position thereby can select between modes with different symmetries. This effect can be used to exert forces on plasmonic structures on the nanometer length scale with great control.

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1.Pelton, M., Aizpurua, J., Bryant, G.W., Laser and Photonics Reviews 2, 136 (2008).
2.Hillenbrand, R., Keilmann, F., Hanarp, P., Sutherland, D.S., Aizpurua, J., Appl. Phys. Lett. 83, 368 (2003).
3.Burresi, M., Kampfrath, T., Oosten, D.v., Prangsma, J.C., Song, B.S., Noda, S., Kuipers, L., Phys. Rev. Lett. 105, 123901 (2010).
4.Koenderink, F.A., Kafesaki, M., Buchler, B.C., Sandoghdar, V., Phys. Rev. Lett. 95, 153904 (2005).
5.Powell, C.J., Swan, J.B., Phys. Rev. 115, 869 (1959).
6.Teng, Y.Y., Stern, E.A., Phys. Rev. Lett. 19, 511 (1967).
7.García de Abajo, F.J., Rev. Mod. Phys. 82, 209 (2010).
8.Kuttge, M., Vesseur, E.J.R., Koenderink, A.F., Lezec, H.J., Atwater, H.A., García de Abajo, F.J., Polman, A., Phys. Rev. B 79, 113405 (2009).
9.Coenen, T., Vesseur, E.J.R., Polman, A., Appl. Phys. Lett. 99, 143103 (2011).
10.Kuttge, M., García de Abajo, F.J., Polman, A., Nano Lett. 10, 1537 (2009).
11.Barnard, E.S., Coenen, T., Vesseur, E.J.R., Polman, A., Brongersma, M.L., Nano Lett. 11, 4265 (2011).
12.Cai, W., Sainidou, R., Xu, J., Polman, A., García de Abajo, F.J., Nano Lett. 9, 1176 (2009).
13.Ritchie, R.H., Phys. Rev. 106 (5), 874 (1957).
14.Batson, P.E., Phys. Rev. Lett. 49, 936 (1982).
15.Ferrell, T.L., Echenique, P.M., Phys. Rev. Lett. 55 (14), 1526 (1985).
16.Bosman, M., Keast, V.J., Watanabe, M., Maaroof, A.I., Cortie, M.B., Nanotechnology 18, 165505 (2007).
17.Nelayah, J., Kociak, M., Stéphan, O., García de Abajo, F.J., Tencé, M., Henrard, L., Taverna, D., Pastoriza-Santos, I., Liz-Marzán, L.M., Colliex, C., Nat. Phys. 3, 348 (2007).
18.Scholl, J.A., Koh, A.L., Dionne, J.A., Nature 483, 421 (2012).
19.Yurtsever, A., van der Veen, R.M., Zewail, A.H., Science 335, 59 (2012).
20.Chu, M.-W., Myroshnychenko, V., Chen, C.H., Deng, J.-P., Mou, C.-Y., García de Abajo, F.J., Nano Lett. 9, 399 (2009).
21.Kuttge, M., Vesseur, E.J.R., Verhoeven, J., Lezec, H.J., Atwater, H.A., Polman, A., Appl. Phys. Lett. 93, 113110 (2008).
22.van Wijngaarden, J.T., Verhagen, E., Polman, A., Ross, C.E., Lezec, H.J., Atwater, H.A., Appl. Phys. Lett. 88 (22), 221111 (2006).
23.Bashevoy, M.V., Jonsson, F., Krasavin, A.V., Zheludev, N.I., Nano Lett. 6 (6), 1113 (2006).
24.Hofmann, C.E., Vesseur, E.J.R., Sweatlock, L.A., Lezec, H., García de Abajo, F.J., Polman, A., Atwater, H.A., Nano Lett. 7, 3612 (2007).
25.Kuttge, M., Vesseur, E.J.R., Polman, A., Appl. Phys. Lett. 94, 183104 (2009).
26.Zhu, X.L., Ma, Y., Zhang, J.S., Xu, J., Wu, X.F., Zhang, Y., Han, X.B., Fu, Q., Liao, Z.M., Chen, L., Yu, D.P., Phys. Rev. Lett. 105, 127402 (2010).
27.Kuttge, M., Cai, W., García de Abajo, F.J., Polman, A., Phys. Rev. B 80, 033409 (2009).
28.Ditlbacher, H., Hohenau, A., Wagner, D., Kreibig, U., Rogers, M., Hofer, F., Aussenegg, F.R., Krenn, J.R., Phys. Rev. Lett. 95, 257403 (2005).
29.Miyazaki, H.T., Kurokawa, Y., Phys. Rev. Lett. 96, 097401 (2006).
30.Novotny, L., van Hulst, N., Nat. Photonics 5, 83 (2011).
31.Vesseur, E.J.R., de Waele, R., Kuttge, M., Polman, A., Nano Lett. 7, 2843 (2007).
32.Vesseur, E.J.R., de Waele, R., Lezec, H.J., Atwater, H.A., García de Abajo, F.J., Appl. Phys. Lett. 92, 83110 (2008).
33.Denisyuk, A.I., Adamo, G., MacDonald, K.F., Edgar, J., Arnold, M.D., Myroshnychenko, V., Ford, J., García de Abajo, F.J., Zheludev, N.I., Nano Lett. 10, 3250 (2010).
34.Kuttge, M., PhD thesis, FOM Institute for Atomic and Molecular Physics, Amsterdam (2009).
35.Vesseur, E.J.R., Garcia de Abajo, F.J., Polman, A., Nano Lett. 9, 3147 (2009).
36.Bozhevolnyi, S.I., Volkov, V.S., Devaux, E., Laluet, J.-Y., Ebbesen, W., Nature 440, 508 (2006).
37.Vesseur, E.J.R., Polman, A., Nano Lett. 11, 5524 (2011).
38.Coenen, T., Vesseur, E.J.R., Polman, A., Koenderink, A.F., Nano Lett. 11, 3779 (2011).
39.Coenen, T., Vesseur, E.J.R., Polman, A., ACS Nano 6, 1742 (2012).
40.Frimmer, M., Coenen, T., Koenderink, A.F., Phys. Rev. Lett. 108, 077404 (2012).
41.Chaturvedi, P., Hsu, K.H., Kumar, A., Fung, K.H., Mabon, J.C., Fang, N.X., ACS Nano 3, 2965 (2009).
42.Takeuchi, K., Yamamoto, N., Opt. Express 19, 12365 (2011).
43.Reyes-Coronado, A., Barrera, R.G., Batson, P.E., Echenique, P.M., Rivacoba, A., Aizpurua, J., Phys. Rev. B 82, 235429 (2010).
44.Prodan, E., Radloff, C., Halas, N.J., Nordlander, P.A., Science 302, 419 (2003).
45.Xu, H., Bjerneld, E.J., Käll, M., Börjesson, L., Phys. Rev. Lett. 83, 4357 (1999).
46.Xu, H., Aizpurua, J., Käll, M., Apell, P., Phys. Rev. E 62, 4318 (2000).
47.Batson, P.E., Surf. Sci. 156, 720 (1985).
48.Batson, P.E., Ultramicroscopy 9, 277 (1982).
49.Yamamoto, N., Araya, K., García de Abajo, F.J., Phys. Rev. B 64, 205419 (2001).
50.Yamamoto, N., Ohtani, S., García de Abajo, F.J., Nano Lett. 11, 91 (2011).
51.Batson, P.E., Reyes-Coronado, A., Barrera, R.G., Rivacoba, A., Echenique, P.M., Aizpurua, J., Nano Lett. 11, 3388 (2011).
52.Vesseur, E.J.R., PhD thesis, FOM Institute AMOLF, Utrecht University (2011).
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