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Porphyrin-based photocatalysts for hydrogen production

Published online by Cambridge University Press:  10 January 2020

Liang Wang ,
Hongyou Fan  and
Feng Bai
Liang Wang
Affiliation:
Henan University, China; chg_2010@qq.com
Hongyou Fan
Affiliation:
Sandia National Laboratories and Department of Chemical and Biological Engineering, The University of New Mexico, USA; hfan@sandia.gov
Feng Bai
Affiliation:
Henan University, China; baifengsun@126.com
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Abstract

Photocatalytic hydrogen production from water is a facile and clean approach to convert rich solar energy into chemical fuel. Developing efficient and robust catalysts to accelerate water-splitting speed is key. Porphyrins exist widely in green plants and are a key photosensitizer to absorb and transfer light energy to other parts of the photosynthesis system of plants. They are considered an ideal model to construct artificial photocatalysts for hot-carrier-mediated hydrogen production. This article discusses recent achievements in constructing porphyrin-based photocatalysts for hydrogen production, including porphyrin molecules, self-assembled porphyrins, metal–organic frameworks, conjugated porphyrin polymers, and hybrid nanomaterial-based photocatalysts. The design and synthesis principles, structure–property relationships, as well as urgent issues to be solved in the future for every type of photocatalyst are also discussed.

Type
Materials for Hot-Carrier Chemistry
Information
MRS Bulletin , Volume 45 , Issue 1: Materials for Hot-Carrier Chemistry , January 2020 , pp. 49 - 56
Copyright
Copyright © Materials Research Society 2020

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