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Cooperative Effects in Strained Polymeric Networks

  • B Deloche (a1), P Sotta (a1) and J Herz (a2)
Abstract

The orientational order generated in a polymer network by an uniaxial stress is probed with NMR. The experiments are performed on an end-linked polydimethylsiloxane network. When a uniaxial force is applied a detailed analysis of the spectrum shows that the segmental motions become uniaxial around constraint direction. This experimental fact is explained by shortrange orientational interactions between chain segments.

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References
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[1] Deloche, B., Beltzung, M., Herz, J., J.PhysoLett. 1982, 43, 763
[2] Samulski, E.T., Polymer 1985, 26, 177
[3] Herz, J., Belkebir, A., Rempp, P.:,Eur.Polym.J. 1973, 9, 1165
[4] Beltzung, M., Picot, C., Rempp, P. and Herz, J., Macromolecules 1982, 15, 1594.
[5] Gronski, W., Stadtler, R., Jacobi, M., Macromolecules 1984, 17, 741
[6] Sotta, P., Deloche, B., to be published in Macromolecules 1990.
[7] Toriumi, H., Deloche, B., Samulski, E.T., Herz, J., Macromolecules 1985, 18, 305.
[8] Sotta, P., Deloche, B., Herz, J., Lapp, A., Durand, D., Rabadeux, J.C., Macromolecules 1987, 20, 2769
[9] Deloche, B., Samulski, E.T., Macromolecules 1988, 21, 3107
[10] Cohen-Addad, J.P., Vogin, R., Phys.Rev.Lett. 1974, 33, 940
[ll] Cohen-Addad, J.P., Domard, M., Lorentz, G., Herz, J., J.Phys (Les Ulis Fr.) 1984, 45, 575
[12] Bastide, J., Leibler, L., Macromolecules 1988, 21, 2647
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MRS Online Proceedings Library (OPL)
  • ISSN: -
  • EISSN: 1946-4274
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