Hostname: page-component-76fb5796d-9pm4c Total loading time: 0 Render date: 2024-04-26T11:54:05.324Z Has data issue: false hasContentIssue false

Laser-Induced Transient Structural Changes in Ag(111) Studied by Time Resolved X-ray Diffraction

Published online by Cambridge University Press:  10 April 2013

Ali Oguz Er*
Affiliation:
Department of Chemistry, University of California, Irvine, CA 92697
Jie Chen
Affiliation:
Key Laboratory for Laser Plasmas (Ministry of Education) and Department of Physics, Shanghai Jiao Tong University, Shanghai 200240, China
Peter M. Rentzepis
Affiliation:
Department of Chemistry, University of California, Irvine, CA 92697
*
*Email: aer@uci.edu
Get access

Abstract

The transient lattice changes on the Ag(111) crystal due to acoustic wave propagation after excitation with femtosecond pulses was studied by means of time resolved X-ray diffraction. The lattice disorder after UV irradiation is detected by changes of the XRD rocking curve shift, broadening, and total diffraction intensity as a function of time. We have observed a blast force formed within two picoseconds after fs UV irradiation. Experimental results show an initial lattice contraction followed by lattice expansion that propagates with sound velocity.

Type
Articles
Copyright
Copyright © Materials Research Society 2013

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

REFERENCES

Falkovsky, L. A., Mishchenko, E. G., Electron-lattice kinetics of metals heated by ultrashort laser pulses, JETP 88, 8488 (1999).CrossRefGoogle Scholar
Chen, J. K., Beraun, J. E., Grames, L. E., and Tzou, D. Y., Short-Time Thermal Effects on Thermomechanical Response Caused By Pulsed Lasers, J. Thermophys. Heat Trans. 17, 3542 (2003).CrossRefGoogle Scholar
Chen, L. X., Jager, W. J. H., Jennings, G., Gosztola, D. J., Munkholm, A., and Hessler, J. P., Capturing a Photoexcited Molecular Structure Through Time-Domain X-ray Absorption Fine Structure, Science 292, 262264 (2001).CrossRefGoogle ScholarPubMed
Tzou, D. Y., Chen, J. K., and Beraun, J. E., Hot electron blast induced by ultrashort-pulsed lasers in layered media, Int. J. Heat Mass. Trans. 45, 33693382 (2002).CrossRefGoogle Scholar
Chen, J., Tomov, I. V., Elsayed-Ali, H. E., Rentzepis, P. M., Hot electrons blast wave generated by femtosecond laser pulses on thin Au(111) crystal, monitored by subpicosecond X-ray diffraction, Chem. Phys. Lett. 419, 374378 (2006).CrossRefGoogle Scholar
Chen, J., Chen, W. -K., Rentzepis, P. M., Blast wave and contraction in Au(111) thin film induced by femtosecond laser pulses. A time resolved x-ray diffraction study, J. Appl. Phys. 109, 113522–5 (2011).CrossRefGoogle Scholar
Er, A. O., Chen, J., Rentzepis, P. M., Ultrafast time resolved x-ray diffraction, extended x-ray absorption fine structure and x-ray absorption near edge structure, J. Appl. Phys. 112, 031101–16 (2012).Google Scholar
Groeneveld, R. H. M., Sprik, R., and Lagendijk, A., Femtosecond spectroscopy of electron-electron and electron-phonon energy relaxation in Ag and Au, Phys. Rev. B 51, 1143311445 (1995).CrossRefGoogle ScholarPubMed
Park, H., Wang, X., Nie, S., Clinite, R., and Cao, J., Mechanism of coherent acoustic phonon generation under nonequilibrium conditions, Phys. Rev. B 72, 100301(R)-4 (2005).CrossRefGoogle Scholar
Tomov, I. V., Chen, J., Ding, X., Rentzepis, P. M., Efficient focusing of hard X-rays generated by femtosecond laser driven plasma, Chem. Phys. Lett. 389, 363369 (2004).CrossRefGoogle Scholar
Park, H., Nie, S., Wang, X., Clinite, R., and Cao, J., Optical Control of Coherent Lattice Motions Probed by Femtosecond Electron Diffraction, J. Phys. Chem. B 109, 1385413856 (2005).CrossRefGoogle ScholarPubMed
Nicoul, M., Shymanovich, U., Tarasevitch, A., von der Linde, D., Sokolowski-Tinten, K., Picosecond acoustic response of a laser-heated gold-film studied with time-resolved x-ray diffraction, Appl. Phys. Lett. 98, 191902–3 (2011).CrossRefGoogle Scholar
Cavalleri, A., Siders, C. W., Brown, F. L. H., Leitner, D. M., Tóth, C., Squier, J. A., Barty, C. P. J., Wilson, K. R., Sokolowski-Tinten, K., Horn von Hoegen, M., von der Linde, D., Kammler, M., Anharmonic Lattice Dynamics in Germanium Measured with Ultrafast X-Ray Diffraction, Phys. Rev. Lett. 85, 586589 (2000).CrossRefGoogle ScholarPubMed
Gan, Y., Chen, J. K., Thermomechanical wave propagation in gold films induced by ultrashort laser pulses, Mechan. Mater. 42, 491501 (2010).10.1016/j.mechmat.2010.01.006CrossRefGoogle Scholar
Chan, W.-L., Averback, R. S., Cahill, D. G., Lagoutchev, A., Dynamics of femtosecond laser-induced melting of silver, Phys. Rev. B 78, 214107–8 (2008).CrossRefGoogle Scholar