Published online by Cambridge University Press: 25 February 2011
Several advances in time-resolved optical measurement techniques have beenmade, which allow a more detailed determination of the optical properties ofsilicon immediately before, during, and after pulsed laser irradiation. Itis now possible to follow in detail the time-resolved reflectivity signalnear the melting threshold; measurements indicate that melting occurs in aspatially inhomogeneous way. The use of time-resolved ellipsometry allowedus to accurately measure the optical properties of the high reflectivity(molten) phase, and of the hot, solid silicon before and after the laserpulse. We obtain n = 3.8, k = 5.2 (±10.1) at λ = 632.8 nm for the highreflectivity phase, in minor disagreement with the published values ofShvarev et al. for liquid silicon. Before and after the high reflectivityphase, the time-resolved ellipsometry measurements are entirely consistentwith the known optical properties of crystalline silicon at temperatures upto its melting point.
Research sponsored by the Division of Materials Sciences, U. S.Department of Energy under contract DE-ACO5-840R21400 with MartinMarietta Energy Systems, Inc.