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  3. Photodissociation Dynamics
  • Cited by 559
      • Reinhard Schinke, Max-Planck-Institut für Strömungsforschung, Göttingen, Germany
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    • Publisher:
      Cambridge University Press
      Publication date:
      15 December 2009
      08 April 1993
      ISBN:
      9780511586453
      9780521484145
      DOI:
      https://doi.org/10.1017/CBO9780511586453
      Dimensions:
      Weight & Pages:
      Dimensions:
      (247 x 174 mm)
      Weight & Pages:
      0.761kg, 436 Pages
      • Subjects:
      Optics, Optoelectronics and Photonics, Physics and Astronomy, Physical Chemistry, Atomic Physics, Molecular Physics and Chemical Physics, Chemistry
      Series:
      Cambridge Monographs on Atomic, Molecular and Chemical Physics (1)
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    • Selected: Digital
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    Subjects:
    Optics, Optoelectronics and Photonics, Physics and Astronomy, Physical Chemistry, Atomic Physics, Molecular Physics and Chemical Physics, Chemistry
    Series:
    Cambridge Monographs on Atomic, Molecular and Chemical Physics (1)
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    Book description

    Photodissociation induced by the absorption of single photons permits the detailed study of molecular dynamics such as the breaking of bonds, internal energy transfer and radiationless transitions. The availability of powerful lasers operating over a wide frequency range has stimulated rapid development of new experimental techniques which make it possible to analyse photodissociation processes in unprecedented detail. This text elucidates the achievements in calculating photodissociation cross-sections and fragment state distributions from first principles, starting from multi-dimensional potential energy surfaces and the Schrödinger equation of nuclear motion. Following an extended introduction in which the various types of observables are outlined, the book summarises the basic theoretical tools, namely the time-independent and the time-dependent quantum mechanical approaches as well as the classical picture of photodissociation. The discussions of absorption spectra, diffuse vibrational structures, the vibrational and rotational state distributions of the photofragments form the core of the book. More specific topics such as the dissociation of vibrationally excited molecules, emission during dissociation, or nonadiabatic effects are also discussed. It will be of interest to graduate students and senior scientists working in molecular physics, spectroscopy, molecular collisions and molecular kinetics.

    Reviews

    ‘Schinke has amply fulfilled his declared aim of providing an overview of the field for graduate students.’

    Source: Nature

    ‘This book is designed to become standard reading for graduate students about to embark on research careers in chemical dynamics.’

    Source: Science

    ‘The material is well prepared, clearly and systematically presented, with numerous instructive figures.’

    Source: Zeitschrift für Physikalische Chemie

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