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A comparison of the intensity scaling for nonlinear Compton scattering and bremsstrahlung X-ray emission

Published online by Cambridge University Press:  23 June 2025

Christina Ingleby*
Affiliation:
York Plasma Institute, University of York , York, UK
Stuart Morris
Affiliation:
Department of Physics, University of Warwick , Coventry, UK
Christopher Arran
Affiliation:
York Plasma Institute, University of York , York, UK
Christopher Ridgers
Affiliation:
York Plasma Institute, University of York , York, UK
Kate Lancaster
Affiliation:
York Plasma Institute, University of York , York, UK
*
Correspondence to: C. Ingleby, York Plasma Institute, University of York, York YO10 5DD, UK. Email: christina.ingleby@york.ac.uk

Abstract

Ultraintense laser–plasma experiments generate a variety of high-energy radiations, including nonlinear inverse Compton scattered (NCS) X-rays, which are expected to be a key experimental observable as we transition into the quantum electrodynamic plasma regime. However, there is also a high bremsstrahlung X-ray background that reduces our ability to observe NCS X-rays. Previous numerical studies comparing NCS and bremsstrahlung emissions fail to capture the full temporal emission of both processes. We present for the first time two-dimensional particle-in-cell (PIC) and three-dimensional hybrid-PIC EPOCH simulations that capture up to 150 ps of the laser–plasma interaction and directly compare the NCS and bremsstrahlung emissions for a plastic target for intensities of ${10}^{20}{-}{10}^{23}$ W/cm2. We present angular distribution plots where the NCS emission is seen to dominate at intensities greater than 5$\times {10}^{21}$ W/cm2 and the target design is seen to successfully divert the bremsstrahlung signal away from the NCS lobe regions, making the experimental observation of nonlinear inverse Compton scattering at lower intensities more likely.

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Type
Research Article
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Creative Common License - CCCreative Common License - BY
This is an Open Access article, distributed under the terms of the Creative Commons Attribution licence (https://creativecommons.org/licenses/by/4.0), which permits unrestricted re-use, distribution and reproduction, provided the original article is properly cited.
Copyright
© The Author(s), 2025. Published by Cambridge University Press in association with Chinese Laser Press

1 Introduction

With the commissioning of new multi-PW laser facilities, laser intensities beyond ${10}^{22}$ W/cm2 are now achievable and open new avenues for investigating high-intensity laser–plasma interactions. These lasers produce strong electromagnetic (EM) fields that accelerate electrons in solid targets to ultra-relativistic energies. As the strength of the electric field approaches the Schwinger limit ( ${E}_\mathrm{S}=1.32\times {10}^{18}$ V/m), the electrons become more relativistic and radiate a significant portion of their energy as X-ray (gamma-ray) photons[ Reference Di Piazza, Muller, Hatsagortsyan and Keitel1 Reference Stark, Toncian and Arefiev4]. The ratio of the laser field compared to the Schwinger limit in the rest frame of the relativistic electrons is defined as the electron quantum parameter ${\chi}_\mathrm{e}$ . It is given by Equation (1); here ${\chi}_\mathrm{e}$ depends on the components of the electric field of the laser (E ${}_{\perp }$ and ${E}_{\parallel }$ ), the velocity of the electrons ( ${\mathbf{v}}_{\mathrm{e}}$ ), the magnetic field of the laser (B) and the electron Lorentz factor ( ${\gamma}_\mathrm{e}$ ):

(1) $$\begin{align}{\chi}_\mathrm{e}=\frac{\gamma_\mathrm{e}}{E_\mathrm{S}}\sqrt{{\left({\mathbf{E}}_{\perp }+{\mathbf{v}}_\mathrm{e}\times \mathbf{B}\right)}^2+{E}_{\parallel}^2/{\gamma}_\mathrm{e}^2}.\end{align}$$

When the electron quantum parameter ${\chi}_\mathrm{e}>0.1$ , quantum and relativistic effects become important and influence classical plasma processes, generating a quantum electrodynamic (QED) plasma[ Reference Ridgers, Brady, Duclous, Kirk, Bennett, Arber, Robinson and Bell5]. QED plasmas are predicted to produce intense high-energy radiation, such as hard X-ray bursts through nonlinear inverse Compton scattering[ Reference Blackburn, Seipt, Bulanov and Marklund6]. Nonlinear inverse Compton scattered (NCS) X-rays are produced when multiple low-energy photons interact with an electron in the presence of a strong EM field, producing a high-energy photon as a result[ Reference Bula, McDonald, Prebys, Bamber, Boege, Kotseroglou, Melissinos, Meyerhofer, Ragg, Burke, Field, Horton-Smith, Odian, Spencer, Walz, Berridge, Bugg, Shmakov and Weidemann7]. High-energy NCS photons also produce electron–positron pairs through the nonlinear Breit–Wheeler (NLBW) process[ Reference Brady, Ridgers, Arber and Bell8]. NCS X-rays, electron–positron pairs and high-energy ions are all relevant to a wide range of applications, including radiography, radiotherapy[ Reference Ledingham and Galster9], laboratory astrophysics and fast ignition fusion schemes[ Reference Culfa and Sert10, Reference Gibbon and Forster11].

Previous simulation work has indicated that the intense bursts of NCS X-rays are a key observable when we transition into the QED plasma regime[ Reference Ridgers, Brady, Duclous, Kirk, Bennett, Arber and Bell12]. However, at currently achievable laser intensities of ${10}^{20}$ ${10}^{22}$ W cm–2, the additional X-ray emission process of bremsstrahlung emission is also present and generates X-rays that are currently indistinguishable from NCS X-rays[ Reference Vyskocil, Klimo and Weber13]. NCS X-rays are rarely observed unambiguously at current laser intensities due to the high bremsstrahlung background produced from laser–plasma interactions. Recent work[ Reference Pirozhkov, Sagisaka, Ogura, Vishnyakov, Shatokhin, Armstrong, Esirkepov, Izquierdo, Pikuz, Hadjisolomou, Alkhimova, Arran, Tsygvintsev, Valenta, Pikuz, Yan, Jeong, Singh, Finke, Grittani, Nevrkla, Lazzarini, Velyhan, Hayakawa, Fukuda, Koga, Ishino, Kondo, Miyasaka, Kon, Nishikino, Nosach, Khikhlukha, Kolesnikov, Ragozin, Gasilov, Kumar, Nejdl, Sasorov, Weber, Margarone, Kato, Korn, Kiriyama, Kondo, Ridgers, Kawachi, Kando and Bulanov14] has shown that it is possible to estimate the bremsstrahlung background by completing a target thickness scan.

With the advancement of laser technology, it is expected that we will soon be able to probe the QED plasma regime experimentally, but this is complicated by the presence of a high bremsstrahlung background that obscures the key observable NCS X-rays. Therefore, methods of reducing the high bremsstrahlung background must be employed. Previous work[ Reference Morris, Robinson and Ridgers15 Reference Smith, Lancaster, Morris and Ridgers19] has highlighted areas of high electron-to-photon conversion efficiency, showing that bremsstrahlung emission depends on parameters such as target composition and density, target thickness and laser intensity. They show that bremsstrahlung emission can be reduced by using a thin target with a low atomic number (Z) for all currently achievable laser intensities. Using a thin, low-Z target will result in the majority of the electron energy being radiated away by electrons refluxing between the target boundaries.

Many other simulation studies[ Reference Wan, Lv, Jia, Sang and Xie20 Reference Galbiati, Formenti, Grech and Passoni23] have been conducted that compare the scaling of both NCS and bremsstrahlung emissions with peak laser intensity, target thickness or target composition. However, most of these studies have been conducted on multi-fs timescales. As the signal from NCS X-rays can be confounded by bremsstrahlung radiation, any simulation studies must consider the full bremsstrahlung emission. Previous work[ Reference Morris, Robinson and Ridgers15, Reference Morris24] has shown that refluxing electrons can produce bremsstrahlung radiation on a multi-ps timescale that is often neglected in simulation studies. We anticipate that bremsstrahlung emission will dominate at lower intensities, and nonlinear inverse Compton scattering will become prominent at intensities above ${10}^{22}$ W cm–2 [ Reference Ji, Pukhov, Nerush, Kostyukov, Shen and Akli25]. However, the scaling of both emissions with intensity on a multi-ps timescale has not been thoroughly investigated. We have limited knowledge of where the crossover between the dominant emission occurs for scenarios where bremsstrahlung reduction methods and longer simulation timescales are considered.

In this paper, we present the results from novel two-dimensional (2D) particle-in-cell (PIC) and three-dimensional (3D) hybrid-PIC EPOCH[ Reference Arber, Bennett, Brady, Lawrence-Douglas, Ramsay, Sircombe, Gillies, Evans, Schmitz, Bell and Ridgers26] simulations investigating the intensity scaling of bremsstrahlung and NCS X-rays on a multi-ps timescale. We have calculated the X-ray conversion efficiencies ( $\eta$ ) of both populations. The simulations directly compare the NCS and bremsstrahlung emissions using a low-Z solid target of dimensions 10.5 μm $\times$ 1 mm $\times$ 1 mm. The laser intensity was increased from 1 $\times$ 10 ${}^{20}$ to 1 $\times$ 10 ${}^{23}$ W/cm2 to capture the full intensity range available at current facilities. This corresponds to a ${\chi}_\mathrm{e}$ range of approximately $2.5\times {10}^{-4}-0.13$ , so we can expect quantum effects to be present at higher intensities.

2 Methodology

The main objective of the simulations presented in this paper is to investigate the intensity scaling of both NCS and bremsstrahlung X-ray emissions and to demonstrate whether detecting NCS emission is viable at current facilities. The work in this paper uses both the PIC code EPOCH[ Reference Arber, Bennett, Brady, Lawrence-Douglas, Ramsay, Sircombe, Gillies, Evans, Schmitz, Bell and Ridgers26] and its hybrid-EPOCH[ Reference Morris, Robinson and Ridgers15] counterpart, which only considers fast electrons accelerated by the laser at the target’s front surface moving through a static background representing the colder bulk target. Simulating laser–plasma interactions using PIC codes provides a useful tool for physics investigations, but is very computationally expensive, particularly when studies need to be conducted on multi-ps timescales. The hybrid-EPOCH counterpart is more computationally efficient, so it can be run on a multi-ps timescale in 3D on clusters with only a few hundred processors.

Hybrid-EPOCH uses electron injection to model the interaction with the laser pulse, and the injected electron properties are based on supposed laser conditions. It can model the evolution of currents and fields within the target due to the motion of the electrons, such as resistivity and Ohmic heating. The hybrid routines also include scattering and collisions between electrons and ions, such as ionization loss and Moller scattering. Additional routines include the photo-electric effect and K- $\alpha$ emission. However, as the code tracks the evolution of parameters only within the target, it is not capable of determining external fields around the target, such as sheath fields. In laser–plasma interactions, electrons are accelerated through the target and leave the bulk material on a faster timescale than the acceleration of ions. This creates a charge separation and produces a sheath field around the target that acts to accelerate the ions in a process called target normal sheath acceleration (TNSA)[ Reference Wilks, Langdon, Cowan, Roth, Singh, Hatchett, Key, Pennington, MacKinnon and Snavely27]. The generation of the sheath field around the target can cause the refluxing of electrons back into the target. In laser–plasma simulations, fast electrons can escape the simulation window through any of the x, y and z boundaries if they possess sufficient energy to overcome the sheath field surrounding the target. Since hybrid-EPOCH cannot model sheath fields, instead the simulation boundaries can be modified to allow electrons to escape or reflux back into the target to model the effects of a sheath field. The escape kinetic energy value associated with the TNSA boundaries can be scaled using ${\kappa}_\mathrm{esc}{a}_0{m}_{\mathrm{e}}{c}^2$ , and electrons that have energies higher than the escape kinetic energy will leave the simulation window. If electrons do not have sufficient energy to escape then they will be refluxed back into the target and will undergo a momentum loss to the sheath field as a result. The momentum loss can be scaled using ${\kappa}_\mathrm{tnsa}{a}_0{m}_{\mathrm{e}}c$ . When electrons are refluxed back into the target they will be scattered and their trajectory will be modified by some angle ${\sigma}_{\Delta \theta }$ . These scaling laws are taken from a previous study on reflux characteristics in 2D PIC simulations[ Reference Morris, Robinson and Ridgers15, Reference Morris28] and have been benchmarked against experiments for laser intensities between 1 $\times {10}^{20}$ and 1 $\times {10}^{22}$ W/cm2. Values for the TNSA boundary characterization parameters ${\kappa}_\mathrm{esc}$ , ${\kappa}_\mathrm{tnsa}$ and ${\sigma}_{\Delta \theta }$ were also determined for different targets at varying intensities.

Figure 1 Schematic of the simulation methodology employed in this paper. The blue rectangle represents the 2D EPOCH simulation domain including a laser and a pre-plasma density gradient. The x = 0 point where the density gradient begins is marked by a solid, black line within the blue rectangle. The green dashed line represents the probe plane that captures electrons leaving the pre-plasma and entering a target. The orange cuboid represents the simulation domain of the 3D hybrid-EPOCH simulation. The TNSA x, y and z boundaries are attached to each face of the orange cuboid within the simulation domain.

The methodology used is shown in Figure 1 and shows a two-stage simulation setup where the laser–plasma interaction is separated. The first step is a 2D EPOCH simulation that captures the laser interaction with the pre-plasma and front surface of the target. The 2D simulation is run on a femtosecond timescale to allow sufficient temporal resolution to capture the full NCS X-ray emission generated. In EPOCH, QED processes such as NCS photon emission, radiation reaction and pair production are modelled using Monte Carlo emission algorithms[ Reference Duclous, Kirk and Bell29, Reference Ridgers, Kirk, Duclous, Blackburn, Brady, Bennett, Arber and Bell30] within the QED module. Multiple species of photons can be initialized independently in the input deck using the identifying tag in each photon species block. This will generate individual outputs for each photon species, including NCS and bremsstrahlung photons. A probe plane is placed behind the front surface of the target to capture the properties of the accelerated electrons as they begin to move through the target material. These electrons are then characterized and converted into a hot electron population that can be injected into a hybrid-EPOCH simulation. The electrons are converted to injectors by assuming cylindrical symmetry and randomly selecting an injection angle between $\pm \pi /2$ to rotate the position and momenta of each electron from the 2D output in the yz plane. This ensures that the electrons are injected within a 3D cone. The particle weight of each electron is then also modified to include the rotation angle and conserve number density within each grid cell. The modified electron population is then injected into a 3D hybrid-EPOCH simulation that captures hot electrons as they traverse the target material, producing bremsstrahlung X-rays as they interact with the background target nuclei. This simulation is run on a multi-ps timescale to ensure that the full bremsstrahlung emission is captured.

The 2D EPOCH simulations used a spatial grid of 26 μm $\times$ 40 μm with a grid cell size of 20 nm. The target had y dimensions of 30 μm and a solid thickness of 0.5 μm. The simulations used a CH plastic foil target (polypropylene) with an electron density of $2.9\times {10}^{29}$ m ${}^{-3}$ , which is approximately 240 ${n}_\mathrm{crit}$ (the classical critical density is $1.2\times {10}^{27}$ m ${}^{-3}$ ). However, the electrons within the simulations will travel at relativistic velocities, so we need to consider the relativistically corrected critical density ${n}_{\mathrm{crit},\gamma }$ . Table 1 provides ${n}_{\mathrm{crit},\gamma }$ values for the laser intensities investigated in this paper. An exponential pre-plasma was attached to the front surface of the target using a density profile of the form ${n}_\mathrm{e}={n}_\mathrm{e}{e}^{\left(x-20\ \mu \mathrm{m}\right)/10\ \mu \mathrm{m}}$ from the x = 0 line until the position of the probe plane in Figure 1. The pre-plasma density range for each simulation is given in Table 1 in units of ${n}_{\mathrm{crit},\gamma }$ . For laser intensities more than 5 × 10 ${}^{21}$ W/cm2, some proportion of the pre-plasma will be relativistically underdense and transparent to the laser. Previous studies[ Reference Brady, Ridgers, Arber, Bell and Kirk31 Reference Nakamura, Koga, Esirkepov, Kando, Korn and Bulanov34] have shown that NCS emission is enhanced in regions of relativistically underdense plasmas, and including a pre-plasma with a long-scale length can increase the NCS conversion efficiency. We have included long-scale-length pre-plasma within the simulations but the effects of relativistic transparency are not directly studied within this paper.

Table 1 The relativistically corrected critical density ( ${n}_{\mathrm{crit},\gamma }$ ) for each simulation presented in this paper and the subsequent range of density in the pre-plasma in units of ${n}_{\mathrm{crit},\gamma }$ .

The bulk C ${}^{6+}$ and H ${}^{+}$ ion densities were set to 1/8 and 1/4 of the electron density, respectively. A second edge population of electrons, C ${}^{6+}$ and H ${}^{+}$ ions, was used to avoid the draining of particles due to open boundaries within the simulation. These populations were confined to $x>20.5\;\mu \mathrm{m}$ and $\mid y\mid >15\;\mu \mathrm{m}$ with their x-max, y-min and y-min boundaries set to be reflective. The initial electron and ion temperatures were set to 1 keV for all simulations. These initial temperatures are insignificant compared to the heating from the laser even in the early stages of the interaction. For simulations below 5 $\times$ 10 ${}^{22}$ W/cm2, 300 ppc (particles per cell) was used for all ion and electron species; 100 ppc was used for 5 $\times$ 10 ${}^{22}$ W/cm2 and 20 ppc was used for 1 $\times$ 10 ${}^{23}$ W/cm2. Convergence tests were conducted at these intensities to evaluate the impact of changing the number of particles per cell and it was found to have a negligible impact. To mitigate unphysical heating in the simulations, current smoothing was used alongside a fifth-order particle shape (BSPLINE3). A 1 μm wavelength laser pulse was focused onto the target surface from the minimum x-boundary at normal incidence. The laser had a Gaussian spatial and temporal profile with full width at half maximum (FWHM) of 5 μm and 40 fs, respectively.

The 3D hybrid-EPOCH simulations used a spatial grid of 10 μm × 1 mm × 1 mm with cell sizes of 70 nm. The carbon and hydrogen densities were set to $3.9\times {10}^{28}$ and $7.7\times {10}^{28}$ m ${}^{-3}$ , respectively. Hybrid-EPOCH assumes a background electron density to enforce neutrality within the bulk target. Any fast electrons that are injected into the simulation will be a small perturbation on top of the assumed electron target density. The initial ion temperatures were set to 300 K (equivalent to 26 $\times {10}^{-3}$ keV) for both species to simulate a cold, dense target. TNSA boundaries were used for both the min and max x, y and z boundaries using the following parameter values: ${\kappa}_\mathrm{esc}=2$ , ${\kappa}_\mathrm{tnsa}=2.7\times {10}^{-3}$ and ${\sigma}_{\Delta \theta}=\pm {23}^{\circ }$ . These are typical values taken from the previous study on refluxing[ Reference Morris, Robinson and Ridgers15, Reference Morris28]. To ensure the full bremsstrahlung emission was captured, the 3D simulations were run for 125 ps.

Figure 2 X-ray photon energy spectra of NCS (blue) and bremsstrahlung (orange) populations from EPOCH simulations for increasing laser intensity up to 1 $\times {10}^{23}$ W/cm2. Note that the axes on the spectra change as the intensity increases to ensure that all of the data can be seen.

3 Results

3.1 Energy spectra

The X-ray photon energy spectra can be seen in Figure 2 and have been plotted using a logarithmic histogram. The data presented in the spectra have been integrated over the entire angular distribution of X-rays. The spectra show low noise for lower photon energies at all intensities, but high shot noise for higher energies. This is to be expected as we anticipate that fewer high-energy photons will be present, but it does present some uncertainty in the results for higher photon energies. For example, in Figure 2(g) there is a small increase in the NCS signal above 300 MeV; however, this is most likely a result of noise in the simulation and will be neglected.

Figure 2 shows that bremsstrahlung emission dominates the energy spectra at most intensities. At lower intensities between 1 $\times {10}^{20}$ and 5 $\times {10}^{21}$ W/cm2, bremsstrahlung emission dominates at most photon energies, particularly at higher energies up to around 50 MeV. However, Figure 2(a) indicates that most of the population is composed of sub-1 MeV photons. The bremsstrahlung emission continues to dominate at higher energies until 3 $\times {10}^{22}$ W/cm2, where nonlinear inverse Compton scattering dominates the entire energy spectrum. Figure 2 indicates that there is a small increase in the total energy and flux of bremsstrahlung emission after nonlinear inverse Compton scattering dominates the spectrum. This can also be seen in Figure 3, a comparison of the bremsstrahlung spectra at some of the highest laser intensities. We can also see that bremsstrahlung emission scales with intensity; however, the change in the total flux and energy decreases as the intensity increases.

Figure 3 Comparison of the bremsstrahlung energy spectra produced from the four highest laser intensities.

Figures 2(a)2(c), show that the NCS photon population has a significantly lower flux and lower total energy than the bremsstrahlung emission and the NCS signal is barely visible on the spectra. We anticipate that nonlinear inverse Compton scattering scales with the laser intensity, and this can be seen from the increase in NCS photon flux and energy as the intensity increases. Figures 2(d) and 2(e) show an increase in the overall NCS photon signal, particularly at lower energies where the signal is higher than the bremsstrahlung signal, although it is not clear at the energies where the NCS signal is higher. When comparing NCS and bremsstrahlung photons directly for all energies, it is difficult to see at which energies nonlinear inverse Compton scattering dominates the spectra at lower intensities. Figure 4 shows spectra for 5 $\times {10}^{21}$ and 1 $\times {10}^{22}$ W/cm2 that have been zoomed in to show photon energies of 0–10 MeV. Figure 4(a) shows that the NCS population dominates the photon spectra for energies up to 2 MeV and that shown in Figure 4(b) dominates up to 10 MeV. These suggest that the NCS photon population consists of a large number of lower-energy photons. In an experimental setting, it would be prudent to focus our attention on characterizing the lower end of the photon spectra where nonlinear inverse Compton scattering is much more abundant than bremsstrahlung emission. This could be done using photon spectrometers that have high-energy resolution below 10 MeV.

Figure 4 Comparison of the energy spectra for photons between 1 keV and 10 MeV for intensities of (a) 5 $\times {10}^{21}$ W/cm2 and (b) 1 $\times {10}^{22}$ W/cm2.

At 3 $\times {10}^{22}$ W/cm2, nonlinear inverse Compton scattering dominates the spectra at all intensities with photon fluxes at least one to two orders of magnitude higher than bremsstrahlung emission and includes photon energies up to 300 MeV. This crossover point where nonlinear inverse Compton scattering dominates is an order of magnitude higher than previous estimates using a 2 μm thick CH target[ Reference Vyskocil, Gelfer and Klimo22]. We expect that our estimate is higher due to using a thicker target and modelling the bremsstrahlung emission up to 125 ps. Previous work has compared nonlinear inverse Compton scattering and bremsstrahlung emission on similar timescales, but this does not capture the full bremsstrahlung emission that will be produced in an experimental setting. It is possible to distinguish between nonlinear inverse Compton scattering and bremsstrahlung emission temporally, but this would require further development of sub-ps photon diagnostics that could provide the necessary temporal resolution (multi-fs) in this instance.

3.2 Angular emission

The photon spectra disguise features that can be measurable in real experiments, where detectors only capture particles emitted in a small angular range. The angular distribution of X-ray energy for nonlinear inverse Compton scattering and bremsstrahlung emission is shown in Figure 5. Here the X-ray energy per radian in the plane ( $\mathrm{dE}/\mathrm{d}\theta$ ) is plotted to allow a direct comparison between the two X-ray populations. The characteristic lobe shape of the NCS emission is seen at $\theta =45$ ° and $\theta =315$ °, or $\pm 45$ ° from the laser propagation axis, and is predominantly in the forward direction, which is consistent with previous studies on NCS emission[ Reference Ridgers, Brady, Duclous, Kirk, Bennett, Arber, Robinson and Bell5, Reference Nakamura, Koga, Esirkepov, Kando, Korn and Bulanov34]. However, other previous studies indicate that these lobes are centred at $\pm 30$ ° from the laser propagation axis.

Figure 5 Two-dimensional angular X-ray energy distribution comparison for nonlinear inverse Compton scattering (blue) and bremsstrahlung emission (orange) for the intensity range ${10}^{20}$ ${10}^{23}$ W/cm2. The laser propagation direction is along the $\theta =0^{\circ}$ axis. Note that the axes in these figures change as the intensity increases to ensure that all of the data can be seen.

Figure 6 Two-dimensional angular energy distribution plot with energy contours for NCS X-ray energies of more than 50 MeV (light blue) and more than 100 MeV (dark blue) for ${10}^{23}$ W/cm2.

NCS emission is small compared to bremsstrahlung emission for intensities up to 5 $\times {10}^{21}$ W/cm2, but becomes the dominant emission at higher intensities. There is a crossover between 5 $\times {10}^{21}$ and 1 $\times {10}^{22}$ W/cm2 where nonlinear inverse Compton scattering begins to dominate, and the emission becomes significantly more prominent at 1 $\times {10}^{22}$ W/cm2. It is much easier to see where nonlinear inverse Compton scattering begins to dominate in the angular profiles than in the energy spectra of Figure 2. Above 1 $\times {10}^{22}$ W/cm2 there is some backward emission (towards $\theta =180$ °), which may be consistent with re-injected electron synchrotron emission (RESE)[ Reference Brady, Ridgers, Arber, Bell and Kirk31] or transversely oscillating electron synchrotron radiation (TOEE)[ Reference Chang, Qiao, Zhang, Xu, Yao, Zhou and He35]. Both processes generate photon emission in the backward direction towards the laser pulse. RESE occurs predominantly in underdense plasma such as that present in the long-scale-length pre-plasma, whereas TOEE occurs in plasma close to near-critical density. The backward emission increases with intensity and, at 3 $\times {10}^{22}$ W/cm2, the backward emission appears to be greater than the forward emission. The backward emission at 1 $\times {10}^{23}$ W/cm2 appears to be of a similar magnitude to the forward emission. However, the evolution of the characteristic lobes requires further investigation. Figure 6 shows the angular distribution for NCS X-rays with KE > 50 MeV and KE > 100 MeV for ${10}^{23}$ W/cm2. The characteristic lobes are still present for higher photon energies but peak at $\pm 30$ °, so the lobes are likely being obscured by an abundance of lower-energy photons in Figure 5. There is still some backward emission present within the 50 MeV contour, which indicates that the backward emission does not only consist of lower-energy photons. However, the majority of emissions for these energy contours are in the forward direction, as expected.

Bremsstrahlung emission dominates at lower intensities, as expected, with the emission becoming more prominent at $\theta =90$ ° and $\theta =270$ ° with increasing intensity. These results are similar to previous studies[ Reference Vyskocil, Klimo and Weber13, Reference Morris, Robinson and Ridgers15] that showed that the angular distribution of bremsstrahlung radiation was affected by changes in the electron momentum components px and py as they reflux across the sheath fields around the target. In the simulations conducted within this paper, when electrons move across the TNSA boundaries they lose energy and momentum due to scattering and so will re-enter the solid with less momentum and energy. We can expect that electrons that pass across the TNSA boundaries more frequently will lose more energy, and thus cannot radiate as much energy through bremsstrahlung emission as they traverse the target. This is the case for electrons moving longitudinally through the target along the laser axis direction as they come into contact with the TNSA x-boundaries more frequently. However, since the target has a larger transverse length, this allows electrons to lose more of their energy through bremsstrahlung radiation before passing through the TNSA y- and z-boundaries[ Reference Morris24]. This produces significant bremsstrahlung emission perpendicular to the laser axis and is directed away from the NCS lobes. Since there is a distinction between the angular emission of both processes, placing X-ray detectors at $\pm 45$ ° on either side of the laser axis would increase the possibility of observing nonlinear inverse Compton scattering experimentally at current facilities.

Figure 7 shows a comparison between the energy spectra for NCS and bremsstrahlung X-rays for angles between 30° and 60° from the laser propagation axis for intensities between ${10}^{21}$ and ${10}^{22}$ W/cm2. It shows the energy spectra we could expect to see by placing a detector within the region where the NCS lobes are most prominent. It indicates that we can observe the NCS signal above the bremsstrahlung background for mid-range intensities in multiple energy ranges. Figures 7(a) and 7(b) show that there is a prominent NCS signal in the keV range that is not apparent in Figures 2(d) and 2(e). This extends to the low MeV range for intensities of mid- ${10}^{21}$ and low- ${10}^{22}$ W/cm2. As anticipated, the NCS signal completely dominates the bremsstrahlung signal at intensities of mid- ${10}^{22}$ W/cm2.

Figure 7 Comparison of the photon spectra for ${10}^{21}{-}{10}^{22}$ W/cm2 between angles of 30° and 60° from the laser propagation axis. The axes have been fixed for comparison and are on a log scale.

3.3 Conversion efficiency

The laser-to-NCS photon conversion efficiencies ( ${\eta}_\mathrm{NCS}$ ) and bremsstrahlung conversion efficiencies ( ${\eta}_\mathrm{br}$ ) were calculated and are presented in Figure 8(a). Overall, both efficiencies increase with the laser intensity (I ${}_\mathrm{L}$ ), and it is clear that NCS emission scales more rapidly with intensity than bremsstrahlung emission so different scaling laws have been applied. A second-order polynomial fit has been used to determine that ${\eta}_\mathrm{NCS}$ scales with I 2, whereas a first-order polynomial was used to determine the ${\eta}_\mathrm{br}$ scaling (approx. $0.5$ I ${}_\mathrm{L}$ ). Previous studies[ Reference Brady, Ridgers, Arber, Bell and Kirk31] have suggested that the power radiated when electrons collide with a counter-propagating laser pulse scales with ${\gamma}^2{E}^2$ . It is known that laser intensity scales with ${E}^2$ so the power radiated by electrons can be assumed to scale with ${I}^2$ . This nonlinear inverse Compton scattering scaling law is consistent with other studies conducted[ Reference Vyskocil, Gelfer and Klimo22, Reference Galbiati, Formenti, Grech and Passoni23, Reference Ji, Pukhov, Nerush, Kostyukov, Shen and Akli25] that suggest ranges of ${\eta}_\mathrm{NCS}\propto {I}^{1.25-2}$ . Bremsstrahlung emission is expected to scale linearly with the hot electron energy and, thus, with the laser energy. For the simulations in this paper, we have adjusted the laser intensity by linearly increasing the energy in the beam; therefore, a linear scaling law is justified. The scaling law used for bremsstrahlung emission is consistent with other studies conducted in the literature that suggest possible intensity scaling laws of ${\eta}_\mathrm{br}\propto {I}^{0.5-1}$ [ Reference Vyskocil, Klimo and Weber13, Reference Smith, Lancaster, Morris and Ridgers19].

Figure 8 (a) Intensity scaling of the energy conversion efficiencies of laser-NCS X-rays and hot electron-bremsstrahlung X-rays. (b) Comparison of the electron energy spectra produced from the electron injectors for 1 $\times {10}^{23}$ W/cm2 when the QED module is on and off. (c) Bremsstrahlung energy spectra for 1 $\times {10}^{23}$ W/cm2 when the QED module is on and off. (d) Bremsstrahlung angular energy plot for 1 $\times {10}^{23}$ W/cm2 when the QED module is on and off.

Figure 8(a) shows that ${\eta}_\mathrm{NCS}$ increases with laser intensity, reaching a peak at 34.81 $\%$ for 1 $\times {10}^{23}$ W/cm2. This is comparable to previous estimates[ Reference Ridgers, Brady, Duclous, Kirk, Bennett, Arber, Robinson and Bell5, Reference Ridgers, Brady, Duclous, Kirk, Bennett, Arber and Bell12, Reference Ji, Pukhov, Nerush, Kostyukov, Shen and Akli25, Reference Nakamura, Koga, Esirkepov, Kando, Korn and Bulanov34, Reference Hadjisolomou, Jeong, Kolenaty, Macleod, Olšovcová, Versaci, Ridgers and Bulanov36] of 3 $\%$ –40 $\%$ for laser intensities of up to 5 $\times {10}^{23}$ W/cm2. These previous studies have also shown that target properties such as density and pre-plasma scale length have a significant impact on photon conversion efficiencies. There is a transition from a bremsstrahlung-dominated regime (1 $\times {10}^{20}$ –5 $\times {10}^{21}$ W/cm2) to an NCS-dominated regime ( $>$ 5 $\times {10}^{21}$ W/cm2) as the laser intensity increases. The crossover around 5 × ${10}^{21}$ W/cm2 is present and consistent with other results presented in this paper.

The bremsstrahlung conversion efficiency ${\eta}_\mathrm{br}$ is higher than ${\eta}_\mathrm{NCS}$ at lower intensities and peaks at 0.68 $\%$ for $3\times {10}^{22}$ W cm–2, which is less than previous estimates[ Reference Morris, Robinson and Ridgers15]. However, the target consists of lower Z material and has a smaller volume than the targets used in those estimates so we expect the conversion efficiency to be smaller. A linear scaling law has been applied to the bremsstrahlung conversion efficiency in the form ${\eta}_\mathrm{br}$ $\propto 0.5$ I ${}_\mathrm{L}$ . The scaling law is shown to be a good fit to the data for intensities up to 1 $\times {10}^{22}$ W/cm2, after which ${\eta}_\mathrm{br}$ plateaus as we enter the NCS-dominated regime. There is also a decrease in ${\eta}_\mathrm{br}$ at 1 $\times {10}^{23}$ W/cm2 compared to ${\eta}_\mathrm{br}$ at 3 $\times {10}^{22}$ and 5 $\times {10}^{22}$ W/cm2. A plateau and decrease in ${\eta}_\mathrm{br}$ at high intensities could be due to QED effects, such as the radiation reaction, as electrons are producing a high flux of high-energy photons. This will result in a decrease in the total energy of the electron population traversing the target producing bremsstrahlung photons.

To determine whether the decrease in ${\eta}_\mathrm{br}$ is due to nonlinear inverse Compton scattering and QED effects, three additional simulations were run with identical parameters except for the absence of the QED module. Turning off the QED module ensures that the simulation runs without NCS emission and reduces the radiation reaction effect on electrons, producing more high-energy electrons that traverse through the solid. Figure 8(b) shows the electron energy spectra containing the population of electrons that were injected into the 3D hybrid-EPOCH simulation for 1 $\times {10}^{23}$ W/cm2. There is a significant difference in the injected electron population when the QED module is turned off; the population of higher energy electrons increases up to energies of 900 MeV, as opposed to 500 MeV when the QED module is used. The total electron energy injected also increases significantly (×3) when the QED module is turned off. The difference in the electron spectra will be due to radiation reaction effects as the electron population produces NCS photons earlier in the interaction. The reduction in high-energy electrons reduces the rate of bremsstrahlung emission, as shown in Figures 8(c) and 8(d), which show the difference in the bremsstrahlung energy spectra and angular emission due to QED effects. Both the energy spectra and the angular emission are enhanced when there are no QED effects. These simulations are shown by the points ‘QED off’ in Figure 8. There is no difference between the ${\eta}_\mathrm{br}$ values at 1 $\times {10}^{22}$ W/cm2. Still, there is a non-negligible difference at higher intensities indicating that nonlinear inverse Compton scattering and QED effects begin to have a significant impact on bremsstrahlung emission at 5 $\times {10}^{22}$ W/cm2. As more energy is being transferred to the NCS population and high-energy photons are produced, the effects of the radiation reaction on the electrons are greater, which means less energy is available to the bremsstrahlung population. The ‘QED-off’ simulations still indicate a plateau in ${\eta}_\mathrm{br}$ after 5 $\times {10}^{22}$ W/cm2, but this is less significant; ${\eta}_\mathrm{br}$ is 0.98 $\%$ and 1.07 $\%$ for QED-off simulations compared to 0.57 $\%$ and 0.41 $\%$ , respectively, for the original simulations. We have noted that there is a difference in the flux and total energy of the injected electron species when the QED module is turned off, which can explain the increase in ${\eta}_\mathrm{br}$ ; however, it does not explain the presence of the plateau. An additional consideration to make is the effect of the sheath boundaries implemented in the 3D hybrid-PIC simulations. The escape energy values are scaled with laser intensity to ensure that electrons with sufficiently high energy can escape the target and simulation window. Those that do not possess sufficiently high energy lose energy to the boundaries and are refluxed back into the target. However, an increase in the total energy and flux of the electron population when the QED module is turned off has not been accounted for and a higher number of electrons could be escaping through the back of the target. A consequence of this is that the very-high-energy electrons could pass through the material without refluxing and interacting with the target material multiple times. This could cause an apparent plateau and decrease in ${\eta}_\mathrm{br}$ , since an increase in laser intensity does not generate an increase in bremsstrahlung photons.

4 Conclusions

The scaling of NCS and bremsstrahlung X-ray emissions in the intensity range 1 $\times {10}^{20}$ –1 $\times {10}^{23}$ W/cm2 has been investigated by conducting 2D PIC and 3D hybrid-PIC EPOCH simulations. For intensities of less than 5 $\times {10}^{21}$ W/cm2 it was found that bremsstrahlung emission generates more photon energy and dominates both the angular energy distribution and the energy spectra. However, the work conducted within this paper suggests that there is a crossover between the dominant emission mechanism occurring at 5 $\times {10}^{21}$ W/cm2 where NCS emission dominates. Here NCS emission produces a higher total photon energy and dominates the angular energy distribution. The characteristic NCS lobe shapes were observed on the angular distribution plots for all intensities at $\pm 45$ ° from the laser propagation axis. These results suggest that the angular NCS emission and bremsstrahlung emission are prominent in different directions and can be exploited experimentally. From the simulations conducted, we found a maximum NCS conversion efficiency ( ${\eta}_\mathrm{NCS}$ ) of 34.81 $\%$ for 1 $\times {10}^{23}$ W/cm2 compared to a maximum bremsstrahlung conversion efficiency ( ${\eta}_\mathrm{br}$ ) of 0.68 $\%$ for $3\times {10}^{22}$ W/cm2. We noted a plateau in the bremsstrahlung conversion efficiency at high intensities and investigated whether it was a result of increased radiation reaction effects as we enter the NCS-dominated regime. Further work on this includes demonstrating these findings experimentally at a high-power laser facility that can achieve intensities above ${10}^{22}$ W/cm2. These effects should be measurable in upcoming experiments, which could observe nonlinear inverse Compton scattering above the bremsstrahlung background and potentially show the impact of the radiation reaction on bremsstrahlung emission.

Acknowledgements

The authors would like to thank the Science and Technology Facilities Council and the Engineering and Physical Sciences Research Council for their funding towards this project, and the continued support of research into QED laser–plasma physics. The authors acknowledge funding from the Engineering and Physical Sciences Research Council [EP/S022430/1]. All simulations within this paper were conducted on the Viking HPC supercomputer cluster at the University of York. The authors are grateful for computational support from the University of York High-Performance Computing Service, Viking and the Research Computing team. The data associated with this investigation can be accessed using https://doi.org/10.15124/aa980a0d-c4a3-4bf7-a092-9835485d5fb5.

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Figure 0

Figure 1 Schematic of the simulation methodology employed in this paper. The blue rectangle represents the 2D EPOCH simulation domain including a laser and a pre-plasma density gradient. The x = 0 point where the density gradient begins is marked by a solid, black line within the blue rectangle. The green dashed line represents the probe plane that captures electrons leaving the pre-plasma and entering a target. The orange cuboid represents the simulation domain of the 3D hybrid-EPOCH simulation. The TNSA x, y and z boundaries are attached to each face of the orange cuboid within the simulation domain.

Figure 1

Table 1 The relativistically corrected critical density (${n}_{\mathrm{crit},\gamma }$) for each simulation presented in this paper and the subsequent range of density in the pre-plasma in units of ${n}_{\mathrm{crit},\gamma }$.

Figure 2

Figure 2 X-ray photon energy spectra of NCS (blue) and bremsstrahlung (orange) populations from EPOCH simulations for increasing laser intensity up to 1$\times {10}^{23}$ W/cm2. Note that the axes on the spectra change as the intensity increases to ensure that all of the data can be seen.

Figure 3

Figure 3 Comparison of the bremsstrahlung energy spectra produced from the four highest laser intensities.

Figure 4

Figure 4 Comparison of the energy spectra for photons between 1 keV and 10 MeV for intensities of (a) 5$\times {10}^{21}$ W/cm2 and (b) 1$\times {10}^{22}$ W/cm2.

Figure 5

Figure 5 Two-dimensional angular X-ray energy distribution comparison for nonlinear inverse Compton scattering (blue) and bremsstrahlung emission (orange) for the intensity range ${10}^{20}$${10}^{23}$ W/cm2. The laser propagation direction is along the $\theta =0^{\circ}$ axis. Note that the axes in these figures change as the intensity increases to ensure that all of the data can be seen.

Figure 6

Figure 6 Two-dimensional angular energy distribution plot with energy contours for NCS X-ray energies of more than 50 MeV (light blue) and more than 100 MeV (dark blue) for ${10}^{23}$ W/cm2.

Figure 7

Figure 7 Comparison of the photon spectra for ${10}^{21}{-}{10}^{22}$ W/cm2 between angles of 30° and 60° from the laser propagation axis. The axes have been fixed for comparison and are on a log scale.

Figure 8

Figure 8 (a) Intensity scaling of the energy conversion efficiencies of laser-NCS X-rays and hot electron-bremsstrahlung X-rays. (b) Comparison of the electron energy spectra produced from the electron injectors for 1$\times {10}^{23}$ W/cm2 when the QED module is on and off. (c) Bremsstrahlung energy spectra for 1$\times {10}^{23}$ W/cm2 when the QED module is on and off. (d) Bremsstrahlung angular energy plot for 1$\times {10}^{23}$ W/cm2 when the QED module is on and off.