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From equilibrium multistability to spatiotemporal chaos in channel flows of nematic fluids

Published online by Cambridge University Press:  09 July 2026

Rahil N. Valani*
Affiliation:
Rudolf Peierls Centre for Theoretical Physics, University of Oxford, Parks Road, Oxford, OX1 3PU, UK
Sumesh P. Thampi
Affiliation:
Rudolf Peierls Centre for Theoretical Physics, University of Oxford, Parks Road, Oxford, OX1 3PU, UK Department of Chemical Engineering, Indian Institute of Technology Madras, Chennai 600036, India
Julia M. Yeomans
Affiliation:
Rudolf Peierls Centre for Theoretical Physics, University of Oxford, Parks Road, Oxford, OX1 3PU, UK
*
Corresponding author: Rahil N. Valani, rahil.valani@physics.ox.ac.uk

Abstract

Content of image described in text.

We investigate channel-confined, nematic liquid crystals using the Beris–Edwards model of nematohydrodynamics. Using strong homeotropic anchoring at the walls, we find multistability, i.e. multiple coexisting states where the uniform nematic state coexists with states having spatially varying scalar nematic order and director fields. When a pressure gradient is applied, flows develop, and the inherent multistability of the system organises a variety of complex dynamics. For low pressure gradients, steady flows are established, and the director fields that emerge from the multistable states at equilibrium correspond to Bowser and Dowser configurations similar to those reported in experiments. An increasing pressure gradient destabilises steady Bowser and Dowser flow states sequentially, leading to unsteady periodic and chaotic regimes featuring cyclical topological transitions, pulsating flows, advecting defects and spatiotemporal chaos. These findings demonstrate that modest variations in the scalar nematic order, as captured by the Beris–Edwards model, can qualitatively modify equilibrium structures and give rise to complex non-equilibrium behaviour in confined nematics – contrasting with the Ericksen–Leslie model, which assumes a constant scalar order parameter. Our key model predictions – multistability, periodically oscillating states and advecting defect-mediated turbulence – can be experimentally investigated in pressure-driven channel flows of nematic fluids.

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© The Author(s), 2026. Published by Cambridge University Press
Figure 0

Figure 1. Coexistence of multiple equilibrium states in channel-confined nematics with strong homeotropic anchoring. (a) Nematic order at the centre of the channel S(0)$S(0)$ as a function of the dimensionless parameter ϵ=K/(CL2)$\epsilon = {K}/({\textit{CL}^2})$. Simulations were performed by varying K$K$ for fixed C=0.1$C=0.1$ and L=20$L=20$. The red line corresponds to a uniform Q$\boldsymbol{Q}$/Bowser (B) state with constant nematic order S(y)=1$S(y)=1$. The blue line shows the variation of S(0)$S(0)$ in a state with varying Q$\boldsymbol{Q}$/Dowser (D). The varying Q$\boldsymbol{Q}$ state has a constant nematic order parameter S0=1−2π2ϵ$S_0=1-2\pi ^2\epsilon$ (dashed blue line) in the bulk of the channel for small ϵ$\epsilon$, whereas strong spatial variations emerge in S(y)$S(y)$ for larger ϵ$\epsilon$. The yellow curve shows the numerically calculated boundary layer thickness δ$\delta$ defined as the length from the boundary where nematic order reaches 95%S0$95\,\%\,S_0$. The yellow dashed curve shows the fit 2δ/L=5ϵ$2\delta /L=5\sqrt {\epsilon }$. (b) Variations in the scalar nematic order S$S$ and nematic orientation θ$\theta$ for the uniform Q$\boldsymbol{Q}$/Bowser (B) state. (c,d) Corresponding plots for the varying Q$\boldsymbol{Q}$/Dowser (D) states for ϵ=0.001$\epsilon =0.001$ and ϵ=0.03$\epsilon =0.03$, respectively. Colour in greyscale indicates the scalar nematic order parameter S$S$. White lines show the director profile θ(y)$\theta (y)$ across the channel. The dimensionless parameter ϵ$\epsilon$ compares the nematic correlation length to the channel width.

Figure 1

Figure 2. Non-equilibrium steady flow states for pressure-driven nematics in a channel. (a) The nematic free energy Fnem$\mathcal{F}_{\textit{nem}}$ as a function of the applied pressure gradient force F$F$ for B (red dots), D$^-$ (blue dots) and D+$^+$ (cyan dots) states. (bd) The evolution of (top) nematic orientation θ$\theta$, (middle) scalar nematic order S$S$ and (bottom) velocity ux$u_x$ for B, D+$^+$ and D$^-$ states, respectively. Bowser states originate from a uniform Q$\boldsymbol{Q}$ state at equilibrium (F=0$F=0$), whereas Dowser states originate from varying Q$\boldsymbol{Q}$ states. The inset in (a) shows an example nematic configuration (S(y)$S(y)$ and θ(y)$\theta (y)$) and velocity field (ux(y)$u_x(y)$) at F=0.001$F=0.001$ for Bowser and Dowser states. Vertical dashed lines in (a) show the locations of instability of the D$^-$ and B states. Other parameters were fixed to C=0.1$C=0.1$, K=0.01$K=0.01$, L=20$L=20$, λ=0$\lambda =0$. Choosing U$U$ to be the maximum velocity results in the following ranges for dimensionless parameters across the range of F$F$ in the plot: Re∈[0,3.5]$Re \in [0,3.5]$, Er∈[0,200]$Er \in [0,200]$, Pe∈[0,0.06]$Pe \in [0,0.06]$ and ϵ=0.001$\epsilon =0.001$.

Figure 2

Figure 3. Transition from steady to unsteady oscillatory states. (ac) From left to right, kymographs of velocity field ux$u_x$, nematic orientation θ$\theta$, scalar nematic order S$S$, and phase-space projection of the dynamics onto the two-dimensional space of global viscous dissipation Fvis$\mathcal{F}_{{vis}}$ and global free energy Fnem$\mathcal{F}_{\textit{nem}}$ (grey curves show transients, whereas black curves show the stable attractor). In (a), F=0.0032$F=0.0032$, where the system relaxes to the D+$^+$ steady state (cyan circle), whereas (b,c) correspond to F=0.00324$F=0.00324$ and F=0.0034$F=0.0034$, respectively, after the onset of oscillations. (d) The period T$T$ of oscillations as a function of proximity to the transition; in the inset, a power-law scaling for the divergence of the form T∝|F−Fc|−1/2$T\propto |F-F_c|^{-1/2}$ is evident. Other parameters of the system are fixed at C=0.1$C=0.1 $, K=0.01$K=0.01 $, L=20$L=20$ and λ=0$\lambda =0$.

Figure 3

Figure 4. Unsteady dynamics in pressure-driven nematic flows. (a) Bifurcation diagram showing peaks in the time series of the global free energy as functions of F$F$ for the unidirectional, pressure-driven flow set-up. Initial flow velocity is zero, S=1$S=1$, and different colours correspond to different initial orientation profiles, with red favouring B states, blue and cyan favouring D$^-$ and D+$^+$ states, respectively, and grey corresponding to random initial orientations. (bd) Kymographs of velocity, nematic orientation, scalar nematic order and phase-space trajectories (transients in grey, and stable attractors in black) for F=0.008,0.012,0.018$F=0.008, 0.012, 0.018$, respectively. Other parameters of the system are fixed at C=0.1$ C=0.1$, K=0.01$K=0.01$, L=20$L=20$ and λ=0$\lambda =0$. Choosing U$U$ to be the maximum velocity results in the following ranges for dimensionless parameters across the range of F$F$ in the plot: Re∈[0,35]$Re \in [0,35]$, Er∈[0,2000]$Er \in [0,2000]$, Pe∈[0,0.6]$Pe \in [0,0.6]$ and ϵ=0.001$\epsilon =0.001$.

Figure 4

Figure 5. Nematohydrodynamics in two-dimensional pressure-driven channel flows. (a) Bifurcation diagram analogous to figure 4(a) for the full two-dimensional equations of motion (2.1)–(2.3). In two-dimensional flows, multistability is observed between different unsteady dynamical states. (b,e) For example, at F=0.0024$F=0.0024$, spatial uniform initial conditions along x$x$ corresponding to a Bowser or a Dowser configuration result in periodic states where the whole channel periodically transitions between a Bowser-like and a Dowser-like state. (c, f) Conversely, if the initial conditions are random, then defects are stabilised by advection along the channel. This results in weakly chaotic flow, as the defect dynamics is not entirely periodic. (d,g) At a higher value F=0.006$F=0.006$, the turbulent flow becomes more prominent through the continuous formation, annihilation and advection of defects. The kymographs in (eg) are shown for a fixed x=50$x=50$. Other parameter values are the same as for figure 4. Choosing U$U$ to be the maximum velocity results in the following ranges for dimensionless parameters across the range of F$F$ in the plot: Re∈[0,18]$Re \in [0,18]$, Er∈[0,1000]$Er \in [0,1000]$, Pe∈[0,0.3]$Pe \in [0,0.3]$ and ϵ=0.001$\epsilon =0.001$.

Figure 5

Figure 6. Figure 6 long description.Topological defects mediate spatially localised Bowser–Dowser transitions in two-dimensional pressure-driven nematic flows. (a) Snapshot from a simulation at F=0.0014$F=0.0014$, with random initial conditions showing defects advecting along the channel. (be) The one-dimensional profiles of nematic director (top), scalar nematic order (middle) and horizontal velocity (bottom) at different locations along the channel near a defect. A Bowser–Dowser transition is obtained in the one-dimensional profile as the defect is traversed spatially.

Figure 6

Figure 7. Steady flow states for pressure-driven nematics in a channel for parameters (a) C=0.1$C=0.1$, K=0.01$K=0.01$, L=20$L=20$, λ=0.2$\lambda =0.2$, (b) C=0.1$C=0.1$, K=0.01$K=0.01$, L=20$L=20$, λ=1$\lambda =1$ and (c) C=0.1$C=0.1$, K=0.1$K=0.1$, L=20$L=20$, λ=0$\lambda =0$. Vertical dashed lines show when the solution branches become unstable. (d,e) Full bifurcation diagrams, where the peaks in the time series of Fnem$\mathcal{F}_{\textit{nem}}$ are plotted as functions of F$F$ for the parameters corresponding to (b) and (c), respectively. Here, initial flow velocity is zero, and different colours correspond to different initial orientation profiles, with red favouring Bowser states, blue and cyan favouring Dowser states, and grey corresponding to random initial orientations.

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