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Linear stability analysis of differentially heated wall-bounded high-pressure transcritical fluids

Published online by Cambridge University Press:  03 November 2025

Marc Bernades*
Affiliation:
Department of Fluid Mechanics, Universitat Politècnica de Catalunya. BarcelonaTech (UPC) , Barcelona 08019, Spain
Francesco Capuano
Affiliation:
Department of Fluid Mechanics, Universitat Politècnica de Catalunya. BarcelonaTech (UPC) , Barcelona 08019, Spain
Lluís Jofre
Affiliation:
Department of Fluid Mechanics, Universitat Politècnica de Catalunya. BarcelonaTech (UPC) , Barcelona 08019, Spain
*
Corresponding author: Marc Bernades, marc.bernades@upc.edu

Abstract

Mixing and heat transfer rates are typically enhanced in high-pressure transcritical turbulent flow regimes. This is largely due to the rapid variation of thermophysical properties near the pseudo-boiling region, which can significantly amplify velocity fluctuations and promote flow destabilisation. The stability conditions are influenced by the presence of baroclinic torque, primarily driven by steep, localised density gradients across the pseudo-boiling line; an effect intensified by differentially heated wall boundaries. As a result, enstrophy levels increase compared with equivalent low-pressure systems, and flow dynamics diverge from those of classical wall-bounded turbulence. In this study the dynamic equilibrium of these instabilities is systematically analysed using linear stability theory. It is shown that under isothermal wall transcritical conditions, the nonlinear thermodynamics near the pseudo-boiling region favour destabilisation more readily than in subcritical or supercritical states; though this typically requires high-Mach-number regimes. The destabilisation is further intensified in non-isothermal wall configurations, even at low Brinkman and significantly low Mach numbers. In particular, the sensitivity of neutral curves to Brinkman number variations, along with the modal and non-modal perturbation profiles of hydrodynamic and thermodynamic modes, offer preliminary insight into the conditions driving early destabilisation. Notably, a non-isothermal set-up (where walls are held at different temperatures) is found to be a necessary condition for triggering destabilisation in low-Mach, low-Reynolds-number regimes. For the same Brinkman number, such configurations accelerate destabilisation and enhance algebraic growth compared with isothermal wall cases. As a consequence, high-pressure transcritical flows exhibit increased kinetic energy budgets, driven by elevated production rates and reduced viscous dissipation.

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JFM Papers
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Creative Common License - CCCreative Common License - BY
This is an Open Access article, distributed under the terms of the Creative Commons Attribution licence (https://creativecommons.org/licenses/by/4.0/), which permits unrestricted re-use, distribution and reproduction, provided the original article is properly cited.
Copyright
© The Author(s), 2025. Published by Cambridge University Press
Figure 0

Figure 1. Sketch of the Poiseuille flow for isothermal (a) and non-isothermal (b) cases.

Figure 1

Figure 2. Base flow profiles of the isothermal cases listed in table 1 for dimensionless streamwise velocity (a) and reduced temperature (b) as a function of wall-normal direction.

Figure 2

Table 1. Base flow cases studied utilising LST. The first group of cases corresponds to symmetric Poiseuille flows with isothermal walls, whereas the second group considers non-isothermal (differentially heated) cases with different cold ($cw$) and hot ($hw$) wall temperatures. Note: $\text{V-1}^{(\star )}$ is covered for isothermal limit analysis and verification in Appendix D.

Figure 3

Figure 3. Base flow in terms of maximum normalised streamwise velocity (a) and temperature (b) as a function of reduced wall temperature and Brinkman number for the cases listed in table 1.

Figure 4

Figure 4. Neutral curves for various Brinkman numbers at (a) subcritical, (b) transcritical and (c) supercritical regimes. The dashed–dotted line represents the isothermal limit (${\textit{Br}} \xrightarrow {} 0$) and the vertical dashed line indicates ${\textit{Re}}_c = 5772$.

Figure 5

Table 2. Critical Reynolds numbers for the flow cases described in § 5.1 obtained from modal stability analysis. Here NI-5 and NI-6 are assessed at ${\textit{Br}} = 5.6 \times 10^{-6}$, i.e. low ${\textit{Br}}$ similar to the isothermal limit (${\textit{Br}} \xrightarrow {}0$).

Figure 6

Figure 5. Perturbation profiles of the most unstable mode at ${\textit{Re}} = 10\,000$ and $\alpha = 1$ along the wall-normal direction for various Brinkman numbers at (a) subcritical, (b) transcritical and (c) supercritical regimes.

Figure 7

Figure 6. Neutral curves of cases (a) NI-1, (b) NI-2 and (c) NI-3 for different Brinkman numbers.

Figure 8

Figure 7. Perturbation profiles of the most unstable mode at ${\textit{Re}} = 10\,000$ along the wall-normal direction for various ${\textit{Br}}$: (a) NI-1 ($\alpha = 0.8$), (b) NI-2 ($\alpha = 1$) and (c) NI-3 ($\alpha = 0.8$) cases.

Figure 9

Figure 8. Perturbation profiles of the most unstable mode for (a) NI-1 at ${\textit{Re}} = 4000$ and $\alpha = 0.8$, (b) NI-2 at ${\textit{Re}} = 4000$ and $\alpha = 1$, and (c) NI-3 at ${\textit{Re}} = 8000$ and $\alpha = 0.8$.

Figure 10

Figure 9. Growth rate contours at ${\textit{Re}}-\alpha$ for (a) NI-5 and (b) NI-6 cases. The neutral curve for NI-5 is highlighted in red.

Figure 11

Figure 10. Perturbation profiles of the most unstable mode at $\alpha = 0.8$ for (a) NI-5 at ${\textit{Re}} = 4000$, (b) NI-6 at ${\textit{Re}} = 4000$, (c) NI-5 at ${\textit{Re}} = 10\,000$, and (d) NI-6 at ${\textit{Re}} = 10\,000$.

Figure 12

Table 3. Summary of kinetic energy budgets ($\times 10^{-4}$) for the 2-D perturbations at ${\textit{Re}} = 10\,000$. Isothermal cases at $\alpha = 1$, non-isothermal NI-1–5 at $\alpha = 0.6$ and NI-2–3-4–6 at $\alpha = 0.8$.

Figure 13

Figure 11. Energy budget terms along the wall-normal direction at ${\textit{Re}} = 10\,000$ for (a) I-2 at ${\textit{Br}} = 0.1$ (left) and ${\textit{Br}} = 0.5$ (right), (b) I-1 (left) and I-3 (right) both at ${\textit{Br}} = 0.5$, (c) NI-1 at ${\textit{Br}} = 0.1$, and (d) NI-3 at ${\textit{Br}} = 0.1$.

Figure 14

Figure 12. Energy budget compressibility effects for (a) the I-2 case at ${\textit{Br}} = 0.01$ (${M\!a}_b = 0.1$ and $U_r = 42.3\, \rm m\,\rm s^{-1}$) and ${\textit{Br}} = 0.5$ (${M\!a}_b = 1.4$ and $U_r = 351\, \rm m\,\rm s^{-1}$) depicting the evolution of ${M\!a}_g$, $u^\prime$, $v^\prime$ and $P^\prime$ along the wall-normal direction. The perturbations are scaled by a factor of $5\times$ for visualisation. For comparison, the subcritical I-1 case (b) is also reported.

Figure 15

Figure 13. Energy terms along the wall-normal direction at ${\textit{Re}} = 10\,000$ for (a) I-1 at ${\textit{Br}} = 0.1$ and ${\textit{Br}} = 0.5$, and (b) NI-1 at ${\textit{Br}} = 0.1$ and NI-5. The baroclinic effect and compressible vortex production are scaled by a factor of $10\times$ for visualisation.

Figure 16

Figure 14. Transient growth envelopes at ${\textit{Re}} = 1000$ and ${\textit{Br}} = 0.5$ for (a) I-1, (b) I-2 and (c) I-3 cases. The resolution range for case I-2 has been limited to $G_{\textit{max}} = 1000$.

Figure 17

Figure 15. Amplification rates for ${\textit{Re}} = 1000$ at $\alpha = 0$ and $\beta = 2$ for (a) I-1, (b) I-2 and (c) I-3 cases. Inset of (b) corresponds to the exponential amplification rate at $\alpha = \beta =1$ for case I-2.

Figure 18

Figure 16. Transient growth envelopes at ${\textit{Re}} = 1000$ and ${\textit{Br}} = 0.1$ for (a) NI-1, (b) NI-2 and (c) NI-3 cases.

Figure 19

Figure 17. Amplification rates for ${\textit{Re}} = 1000$ at $\alpha = 0$ and $\beta = 2$ for (a) NI-1, (b) NI-2 and (c) NI-3 cases.

Figure 20

Figure 18. Transient growth envelopes at ${\textit{Re}} = 1000$ and ${\textit{Br}} = 5.6 \times 10^{-6}$ for (a) NI-5 and (b) NI-6 cases.

Figure 21

Figure 19. Transient growth envelopes at $\beta = 0$ and ${\textit{Br}} = 0.5$ for (a) I-1, (b) I-2 and (c) I-3 cases with $10$ spaced contour levels. Grey-filled circles denote infinite energy growth. The resolution range for cases I-1 and I-2 has been limited to $G_{\textit{max}} = 5000$.

Figure 22

Figure 20. Transient growth envelopes at $\beta = 0$ and ${\textit{Br}} = 0.1$ for (a) NI-1, (b) NI-2 and (c) NI-3 cases, and ${\textit{Br}} = 5.6 \times 10^{-6}$ for (d) NI-5. The resolution range has been limited to $G_{\textit{max}} = 1000$.

Figure 23

Table 4. Energy-based critical Reynolds numbers and energy growths for the flow cases listed in § 5.1 at two-parameter space $(\alpha , \beta )$ levels. Cases I-1, I-2 and I-3 are assessed at ${\textit{Br}} = 0.5$, NI-1, NI-2, NI-3 and NI-4 at ${\textit{Br}} = 0.1$, and NI-5 and NI-6 at ${\textit{Br}} = 5.6 \times 10^{-6}$. Transition criteria defined if energy grows beyond elapsed time ($t \leqslant 400$), highlighting with superscript $(\boldsymbol{\cdot })^\star$ the exponentially algebraic growth.

Figure 24

Figure 21. Optimum input perturbation profiles at ${\textit{Re}} = 1000$, $\alpha = 0$ and $\beta = 2$ for the isothermal flow cases (a) I-1, I-2 and I-3 at ${\textit{Br}} = 0.5$, (b) NI-1, NI-2 and NI-3 at ${\textit{Br}} = 0.1$, and (c) NI-4 and NI-5 at ${\textit{Br}} = 5.6 \times 10^{-6}$. Results are normalised by $w^\prime$ for all cases.

Figure 25

Figure 22. Optimum output response at ${\textit{Re}} = 1000$, $\alpha = 0$ and $\beta = 2$ for the isothermal flow cases (a) I-1, I-2 and I-3 at ${\textit{Br}} = 0.5$, (b) NI-1, NI-2 and NI-3 at ${\textit{Br}} = 0.1$, and (c) NI-5 and NI-6 at ${\textit{Br}} = 5.6 \times 10^{-6}$. Results are normalised by $u^\prime$ for (a) and $\rho ^\prime$ for (b,c).

Figure 26

Figure 23. Optimum (a) perturbation and (b) response at ${\textit{Re}} = 1000$, $\alpha = \beta = 1$ for the isothermal flow case I-2 at ${\textit{Br}} = 0.5$. Results are normalised by $w^\prime$ for (a) and $\rho ^\prime$ for (b).

Figure 27

Figure 24. Optimum velocity perturbation at ${\textit{Re}} = 1000$, $\alpha = 0$ and $\beta = 2$ for cases (a) I-1 at ${\textit{Br}} = 0.5$, (b) NI-1 at ${\textit{Br}} = 0.1$, and (c) NI-5 at ${\textit{Br}} = 5.6 \times 10^{-6}$.

Figure 28

Figure 25. Optimum response at ${\textit{Re}} = 1000$, $\alpha = 0$ and $\beta = 2$ for (a,b,c) I-1 at ${\textit{Br}} = 0.5$, (d,e,f) NI-1 at ${\textit{Br}} = 0.1$, and (g,h,i) NI-5 at ${\textit{Br}} = 5.6 \times 10^{-6}$.

Figure 29

Figure 26. (a) Disturbed energy over time based on initial optimal input perturbation from transient growth results at ${\textit{Re}}_b = 4000$, $\alpha = 0$ and $\beta = 2$ comparing DNS with the non-modal energy growth, and (b) wall-normal ensemble average of normalised DNS disturbed energy.

Figure 30

Figure 27. Wall-normal vorticity on a $y{-}z$ plane indicating the location of the pseudo-boiling line (purple dashed-doted line) and cross-velocity vector fields for (a) $t^\star \approx 0$, (b) $t^\star \approx 1$ and (c) $t^\star \approx 40$.

Figure 31

Figure 28. Thermodynamic and transport properties of nitrogen at $P/ P_c = 2$ with a temperature range from $T / T_c = 0.75$ to $T / T_c = 1.5$ for NIST, CoolProp and Model (Peng-Robinson equation of state with Chung et al. (1984, 1988) high-pressure coefficients) for density $\rho$, dynamic viscosity $\mu $, isobaric heat capacity $c_p$ and thermal conductivity $\kappa$.

Figure 32

Figure 29. Low-pressure $P/P_c = 0.03$ non-isothermal base flow with a temperature range from $T / T_c = 0.75$ to $T / T_c = 1.5$ utilising nitrogen from (i) ensemble-averaged DNS high-pressure transcritical channel flow, and (ii) linear stability solver for velocity, temperature, dynamic viscosity and thermal conductivity. Both frameworks utilise the thermodynamic model of Peng-Robinson equation of state and Chung et al. (1984, 1988) high-pressure transport coefficients.

Figure 33

Figure 30. Grid convergence results for case I-1 of maximum growth rate modal analysis at $\alpha = 1.0$, ${\textit{Br}} = 0.1$ and ${\textit{Re}} = 10\,000$ (a), and maximum transient growth non-modal analysis at $\alpha = 0.0$, $\beta = 2.0$, ${\textit{Br}} = 0.1$ and ${\textit{Re}} = 1000$ (b).

Figure 34

Figure 31. Operator sensitivity of the wall temperature (a) and bulk pressure (b) for the maximum growth rate for case I-1 at $\alpha = 1.0$, ${\textit{Br}} = 0.1$ and ${\textit{Re}} = 10\,000$.

Figure 35

Figure 32. (a) Eigenspectrum at ${\textit{Re}} = 10\,000$ and wavenumber $\alpha = 1$ and (b) neutral curve. Real-gas framework with CoolProp thermodynamic and transport properties model (RG), ideal gas with power law (IG) and incompressible framework (IC). In (a) the red highlighted eigenvalue corresponds to an unstable mode ($\omega = 0.2375 + 0.0037i$), whereas dark yellow corresponds to a stable mode ($\omega = 0.4164 - 0.1382i$) whose perturbations are depicted in figure 33.

Figure 36

Figure 33. Perturbation profiles of (a) the unstable mode ($\omega = 0.2375 + 0.0037i$) and (b) the stable mode ($\omega = 0.4164 - 0.1382i$) normalised by $| u^{\prime }|$. Real-gas framework with CoolProp thermodynamic and transport properties model (RG) depicted by solid lines, and ideal gas with power law (IG) with markers.

Figure 37

Figure 34. Transient growth map at incompressible conditions (${\textit{Br}} \approx 0$) for ${\textit{Re}} = 2000$.

Figure 38

Figure 35. Optimum eigenvector profiles at incompressible conditions (${\textit{Br}} \approx 0$) for ${\textit{Re}} = 2000$ at maximum growth ($\alpha = 0$ and $\beta = 2$) for (a) input and (b) output. Results are normalised by (a) $w^\prime$ and (b) $u^\prime$.

Figure 39

Figure 36. Transient growth maps at ${\textit{Re}} = 1000$ and ${\textit{Br}} = 0.07$ for CO$_2$ at isothermal conditions with (a) $T = 290\thinspace \textrm {K}$, (b) $T = 300\thinspace \textrm {K}$ and (c) $T = 310\thinspace \textrm {K}$.