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Ultrafast dynamics of a spin-polarized electron plasma with magnetic ions

Published online by Cambridge University Press:  07 January 2025

Benjamin Bakri
Affiliation:
Université de Strasbourg, CNRS, Institut de Physique et Chimie des Matériaux de Strasbourg, UMR7504, F-67000 Strasbourg, France
Nicolas Crouseilles
Affiliation:
Université de Rennes, Inria Rennes (Mingus team) and IRMAR UMR CNRS 6625, F-35042, Rennes, France
Paul-Antoine Hervieux
Affiliation:
Université de Strasbourg, CNRS, Institut de Physique et Chimie des Matériaux de Strasbourg, UMR7504, F-67000 Strasbourg, France
Xue Hong
Affiliation:
Department of Radiation Oncology, University of Kansas Medical Center, KA, USA
Giovanni Manfredi*
Affiliation:
Université de Strasbourg, CNRS, Institut de Physique et Chimie des Matériaux de Strasbourg, UMR7504, F-67000 Strasbourg, France
*
Email address for correspondence: giovanni.manfredi@ipcms.unistra.fr

Abstract

We construct a mean-field model that describes the nonlinear dynamics of a spin-polarized electron gas interacting with fixed, positively charged ions possessing a magnetic moment that evolves in time. The mobile electrons are modelled by a four-component distribution function in the two-dimensional phase space $(x,v)$, obeying a Vlasov–Poisson set of equations. The ions are modelled by a Landau–Lifshitz equation for their spin density, which contains ion–ion and electron–ion magnetic exchange terms. We perform a linear response study of the coupled Vlasov–Poisson–Landau–Lifshitz (VPLL) equations for the case of a Maxwell–Boltzmann equilibrium, focussing in particular on the spin dispersion relation. Conditions of stability or instability for the spin modes are identified, which depend essentially on the electron spin polarization rate $\eta$ and the electron–ion magnetic coupling constant $K$. We also develop an Eulerian grid-based computational code for the fully nonlinear VPLL equations, based on the geometric Hamiltonian method first developed by Crouseilles et al. (J. Plasma Phys., vol. 89, no. 2, 2023, p. 905890215). This technique allows us to achieve great accuracy for the conserved quantities, such as the modulus of the ion spin vector and the total energy. Numerical tests in the linear regime are in accordance with the estimations of the linear response theory. For two-stream equilibria, we study the interplay of instabilities occurring in both the charge and the spin sectors. The set of parameters used in the simulations, with densities close to those of solids (${\approx }10^{29}\ {\rm m}^{-3}$) and temperatures of the order of 10 eV, may be relevant to the warm dense matter regime appearing in some inertial fusion experiments.

Information

Type
Research Article
Creative Commons
Creative Common License - CCCreative Common License - BY
This is an Open Access article, distributed under the terms of the Creative Commons Attribution licence (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted re-use, distribution and reproduction, provided the original article is properly cited.
Copyright
Copyright © The Author(s), 2025. Published by Cambridge University Press
Figure 0

Figure 1. Schematic view of the physical system under consideration. The immobile ions (red circles) provide the main source of localized magnetism. They interact through magnetic exchange both with themselves (coupling constant $J$) and with the itinerant electrons, represented by green dots (coupling constant $K$).

Figure 1

Figure 2. Magnon frequency $\omega _s$ for different normalized magnetic coupling constants $\tilde {K}$, obtained from (3.22) (continuous lines, red for the real part of the frequency, blue for the imaginary part), for $k=0.5$ and $\eta =\tanh (H\tilde {K})$. Note that the electron spin polarization $\eta$ is different for different values of $\tilde {K}$. The dots represent numerical results obtained with the full numerical code described in the forthcoming sections. For this self-consistent case, the imaginary part remains very small with respect to the real part of the frequency.

Figure 2

Figure 3. Magnon frequency $\omega _s$ for different normalized magnetic coupling constants $\tilde {K}$, obtained from (3.22) (continuous lines, red for the real part of the frequency, blue for the imaginary part), for wavenumber $k=0.5$ and electron polarizations (a) $\eta =0.5$ and (b) $\eta =-0.5$. The dots represent numerical results obtained with the full numerical code described in the forthcoming sections. According to the value of $\eta$, the system is either (a) stable or (b) unstable.

Figure 3

Figure 4. Magnon frequency $\omega _s$ as a function of the magnetic coupling constant $\tilde {K}$, for the self-consistent case $\eta = \tanh (H\tilde {K})$, and wavenumber $k=0.5$. The solid lines represent the full dispersion relation computed numerically using (3.22), while the dashed lines are obtained with the simplified relation (3.24). Red lines refer to the real part of $\omega _s$, whereas blue lines refer to the imaginary part.

Figure 4

Figure 5. Magnon frequency $\omega _s$ as a function of the magnon wavenumber $k$, for electron polarization $\eta = 0.5$, and magnetic coupling constant $\tilde {K}=0.16$. The solid lines represent the full dispersion relation computed numerically using (3.22) where the integral and the derivative are not with respect to $\tilde {K}$ but $k$. The other lines refer to the approximate linear theory obtained from (3.23) at first order (dashed lines, given explicitly by (3.24)), and second order (dotted lines). Red lines refer to the real part of $\omega _s$, whereas blue lines refer to its imaginary part.

Figure 5

Table 1. Main numerical and physical parameters of the three runs that use a Maxwell–Boltzmann (MB) equilibrium: initial electron spin polarization $\eta$, ion spin frequency $\omega _s$ and initial perturbation $\varepsilon$. The values of $\omega _s$ are those of the linear response calculation using the ZEAL code. Other values are $k=0.5$, $N_x=119$, $N_v=1024$ and $v_{\max }=5$.

Figure 6

Figure 6. MB1 simulation. Time history of the square root of the electric energy ${\mathcal {H}}_E^{1/2}$ (given by (4.2)), (a) in semi-$\log$ scale and (b) corresponding frequency spectrum. The red straight line represents the linear damping rate given in (5.2). Time history of the absolute value of the real part of the first Fourier mode of the ion spin $\hat {S}_1(k,t)$ in (c) semi-$\log$ scale and (d) corresponding frequency spectrum. The red straight line corresponds to zero damping, see (5.3). The arrows in the spectral plots correspond to the results of linear response theory.

Figure 7

Figure 7. MB2 simulation ($\eta =0.5$). Time history of the absolute value of the real part of the first Fourier mode of the ion spin $\hat {S}_1(k,t)$ (a) in semi-$\log$ scale and (b) corresponding frequency spectrum. The slope of the red straight line is $-0.005186$, very close to the linear response result given in table 1. The peak of the frequency spectrum also matches the linear result $\textrm {Re}\, \omega _s = 0.02088$ (indicated by an arrow on the plot) with good accuracy. Panels (c,d) show the same quantities for the electronic spin mode $\hat {M}_1(k,t)$. The real and imaginary parts of the frequency are the same as for the ion spins.

Figure 8

Figure 8. MB3 simulation ($\eta =-0.5$). Time history of the absolute value of the real part of the first Fourier mode of the ion spin $\hat {S}_1(k,t)$ (a) in semi-$\log$ scale and (b) corresponding frequency spectrum. The slope of the red straight line is $0.00607$, very close to the linear response result given in table 1. The peak of the frequency spectrum also matches the linear result $\textrm {Re} \omega _s = 0.01725$ (indicated by an arrow on the plot) with good accuracy. Panels (c,d) show the same quantities for the electronic spin mode $\hat {M}_1(k,t)$. The real and imaginary parts of the frequency are the same as for the ion spin.

Figure 9

Table 2. Main numerical and physical parameters of the runs that use a two-stream equilibrium. Other values are $k=0.2$ and $N_x=129$.

Figure 10

Figure 9. TS1 simulation. (a) Time evolution of the square root of the electric energy ${\mathcal {H}}_E^{1/2}$ (given by (4.2)) for short times $t\in [0, 50]$. (b) Time evolution of the absolute value of the real part of the fundamental mode of the electron spin $\hat {M}_1$. (c) Time evolution of the absolute value of the real part of the fundamental mode of the ion spin $\hat {S}_1$. The red straight lines have slopes equal to zero for the electric energy and $-6.3 \times 10^{-4}$ for $\hat {M}_1$ and $\hat {S}_1$.

Figure 11

Figure 10. TS2 simulation. (a) Time evolution of the square root of the electric energy ${\mathcal {H}}_E^{1/2}$ (given by (4.2)) for short times $t\in [0, 100]$. (b) Time evolution of the absolute value of the real part of the fundamental mode of the electron spin $\hat {M}_1$. (c) Time evolution of the absolute value of the real part of the fundamental mode of the ion spin $\hat {S}_1$. The red straight lines have slopes equal to $0.2845$ for the electric energy and $4\times 10^{-5}$ for $\hat {S}_1$.

Figure 12

Figure 11. TS3 simulation. (a) Time evolution of the square root of the electric energy ${\mathcal {H}}_E^{1/2}$ (given by (4.2)) for short times $t\in [0, 100]$; the red straight line has slope equal to $0.2845$. (b) Time evolution of the absolute value of the real part of the fundamental mode of the electron spin $\hat {M}_1$. (c) Time evolution of the absolute value of the real part of the fundamental mode of the ion spin $\hat {S}_1$.

Figure 13

Figure 12. TS3 simulation. Contour plots of the distribution functions in the $(x,v)$ phase space at the final time $\omega _p t=10^4$: (a) $f_0$; (b) $f_1$; (c) $f_2$ and (d) $f_3$.

Figure 14

Figure 13. TS4 simulation. (a) Time evolution of the square root of the electric energy ${\mathcal {H}}_E^{1/2}$ (given by (4.2)) for short times $t\in [0, 100]$. (b) Time evolution of the absolute value of the real part of the fundamental mode of the electron spin $\hat {M}_1$. (c) Time evolution of the absolute value of the real part of the fundamental mode of the ion spin $\hat {S}_1$. The red straight lines have slope equal to $0.004$.