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Flow regimes in a melting system composed of binary fluid: transition from penetrative convection to diffusion

Published online by Cambridge University Press:  25 October 2024

Zhong-Han Xue
Affiliation:
State Key Laboratory for Strength and Vibration of Mechanical Structures, School of Aerospace, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, PR China
Jie Zhang*
Affiliation:
State Key Laboratory for Strength and Vibration of Mechanical Structures, School of Aerospace, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, PR China
Ming-Jiu Ni
Affiliation:
School of Engineering Science, University of Chinese Academy of Sciences, Beijing 101408, PR China
*
Email address for correspondence: j_zhang@xjtu.edu.cn

Abstract

In a horizontally heated melting system, where a solid substance is subject to melting by a warmer liquid beneath, the presence of solute in the liquid introduces a complex interplay between temperature and concentration dynamics. Employing a recently developed sharp interface method (Xue et al., J. Comput. Phys., vol. 491, 2023), we conduct direct numerical simulations to investigate the transient behaviour of the system across a broad range of Rayleigh numbers and solute concentrations. Our observations reveal distinct flow regimes: at low concentrations, the system resembles a temperature-driven melting problem, characterized by vortex rolls beneath the melting interface. As the solute concentration increases, a stably stratified layer emerges beneath the interface, leading to the transition from thermal convection to penetrative convection, which resembles those flow characteristics observed in the double-diffusive convection. This shift results from the competition between the stabilizing effect induced by solute concentration gradient and the destabilizing effect caused by temperature gradient. Otherwise in the diffusion regime, characterized by very high solute concentrations, the flow becomes static due to the complete suppression of convection by the stably stratified layer. This regime further exhibits two distinct patterns: ‘melting’ and ‘dissolution’. Beyond characterizing diverse flow patterns, our study conducts a quantitative analysis, examining heat/mass transfer, melting rates, and the evolution of temperature and concentration at the interface. These insights contribute to a better understanding of the intricate interplay between temperature and solute concentration during phase change, with implications for accurately estimating melting rates in binary fluid systems.

Information

Type
JFM Papers
Creative Commons
Creative Common License - CCCreative Common License - BY
This is an Open Access article, distributed under the terms of the Creative Commons Attribution licence (http://creativecommons.org/licenses/by/4.0), which permits unrestricted re-use, distribution and reproduction, provided the original article is properly cited.
Copyright
© The Author(s), 2024. Published by Cambridge University Press.
Figure 0

Figure 1. Schematic illustration of the melting problem involving a binary fluid. (a) The initial configuration for the simulations. (b) The evolving stage of the system. The significance of the symbols in the images is explained in the text.

Figure 1

Figure 2. Flow patterns exhibited by the binary fluid melting system. (a) The distribution of these flow patterns on a phase map of $(Ra, {\varLambda })$ investigated in this study. The inset provides a magnified view of the region $1 \leqslant {\varLambda } \leqslant 10$ for improved visualization. The green dotted line at ${Ra} \approx 1.62 \times 10^5$ marks the threshold for the onset of RBC at the beginning of the simulation, estimated based on the critical Rayleigh number ${Ra}_{{cr}} \approx 1295.78$ derived by Vasil & Proctor (2011). Sketches of (b) the convection regime, (c) the layering regime, and (d) the diffusion regime are provided for clarity.

Figure 2

Figure 3. Characteristics of the convection regime at $(Ra, {\varLambda }) = (10^6, 10^{-2})$. (a) Snapshots of the temperature field (left-hand image), the concentration field (right-hand image), and the solid–liquid interfaces (white solid lines) at different times: $t = 5\times 10^{-3}, 0.1, 0.3, 0.6$. (bd) Time evolution of the horizontally averaged (b) temperature $\tilde {\theta }$, (c) concentration $\tilde {\phi }$, and (d) effective density $\tilde {\rho }$ along the vertical direction $z$. Here, $\tilde {\theta }$, $\tilde {\phi }$ and $\tilde {\rho }$ denote the averaged values at a given $z$. The red portion of a single line represents the liquid phase, while the purple portion indicates the solid phase, with the gradient depicting the presence of a wavy interface at this height. The insets of (b) and (c) present sharp temperature and concentration profiles within the slice $x=2$ at $t=0.48$, revealing interfacial values $\theta _\varGamma \approx 0$ and $\phi _\varGamma \approx 0.2$, discussed further in § 4.2.

Figure 3

Figure 4. Influences of ${\varLambda }$ in the convection regime while maintaining the Rayleigh number at $Ra = 10^6$. (a) Temporal evolution of the temperature distribution located at $(x,\bar {h}(t)/2)$, with ${\varLambda }$ varied between $0.1$, $0.5$ and $1$. The white dotted line indicates the occurrence of the first cell merging in each case. (a) Images reveal that a larger ${\varLambda }$ leads to earlier cell merging. Contour maps of (b) solute concentration and (c) temperature are shown at $t = 0.228$ for ${\varLambda } = 1$. Comparing (b,c) indicates that thermal plumes are launched from positions where fresher plumes are located.

Figure 4

Figure 5. Snapshots depicting the temperature field (left-hand images), the concentration field (right-hand images), and the positions of the solid–liquid interfaces (illustrated by white solid lines) within the diffusion regime. These snapshots correspond to scenarios at (a) $(Ra, {\varLambda }) = (10^6, 5)$ and (b) $(Ra, {\varLambda }) = (10^6, 10^3)$. The progression of time is displayed from bottom to top: $t = 10^{-2}$, $5\times 10^{-2}$ and $1$.

Figure 5

Figure 6. Temporal evolution of the horizontally averaged (a,c,e) temperature and (b,df) concentration in the vertical direction, maintaining $Ra = 10^6$ and varying ${\varLambda }$ between $5, 10^2, 10^3$. The descriptions are consistent with those of figure 3. It is evident that at ${\varLambda } = 5$, the temperature remains nearly constant at $\tilde {\theta } = 0$ within the solid, while becoming linearly distributed across the entire domain at ${\varLambda } > 10^2$. Concerning the concentration, a higher ${\varLambda }$ leads to a more pronounced discontinuity of $\tilde {\phi }$ at the interface.

Figure 6

Figure 7. Characteristics of the layering regime with penetrative convection at $(Ra, {\varLambda }) = (10^7, 3)$. (a) Snapshots of the temperature field (left-hand image), concentration field (right-hand image) and solid–liquid interfaces (indicated by white solid lines) at times $t = 10^{-2}$, $0.1$, $0.5$ and $1.5$, from bottom to top. (bd) The time evolutions of the vertical distribution of the averaged temperature, concentration and density at a given height, respectively. Descriptions are consistent with those provided in figure 3. (e) The time evolution of the averaged local density ratio along the height, $\widetilde {{\varLambda }^*}(z,t)$, in the $(t,z)$ plot, with the blue solid line denoting the position of the solid–liquid interface.

Figure 7

Figure 8. Characteristics of the layering regime with convection–convection double-layer structure at $(Ra, {\varLambda }) = (10^8, 3)$, with descriptions identical to those in figure 7, except that the time moments of the snapshots in (a) are $t=10^{-2}$, 0.1, 0.3 and $0.5$ from bottom to top.

Figure 8

Figure 9. The temporal evolution of (a) the thermal Nusselt number ${Nu}_T(t)$ and (b) the solutal Nusselt number ${Nu}_C(t)$, plotted against ${Ra}_e(t)$ for varying $Ra$ (${Ra}=10^6,10^7,10^8$) and ${\varLambda }$ ($10^{-2} \leqslant {\varLambda } \leqslant 10^3$). In (b), the dash-dotted line represents the predicted value of ${Nu}_C\approx 2.49$ for the ‘melting’-dominated diffusion regime (${\varLambda } \leqslant 10$) obtained through scaling analysis. For better readability, the different groups of profiles with ${Ra}=10^6$, $10^7$ and $10^8$ are distinguished by different transparency. Also, the range of ${Ra}_e$ for different ${Ra}$ is highlighted in both plots.

Figure 9

Figure 10. Time evolution of $\bar {\phi }_\varGamma (t)$ within the range of small to moderate ${\varLambda }$ (${\varLambda } \leqslant 10$) depicted at (a) ${Ra=10^6}$, (b) ${Ra}=10^7$, and (c) ${Ra}=10^8$, respectively. The corresponding ${\varLambda }$ values are represented by different line colours, consistent with those in figure 9. (d) The ultimate value of $\bar {\phi }_\varGamma$ as a function of ${\varLambda }$ for different ${Ra}$. (e) A schematic representation of the one-dimensional BL-shortcut-BL structure for the concentration $\phi$ and temperature $\theta$ profiles. The upper and lower solutal (thermal) boundary layers are symbolized by $\delta _{\phi,u}$ and $\delta _{\phi,\ell }$ ($\delta _{\theta,u}$ and $\delta _{\theta,\ell }$), respectively.

Figure 10

Figure 11. Evolution of the averaged interfacial values of temperature $\bar {\theta }_\varGamma$ and concentration $\bar {\phi }_\varGamma$ in the ‘dissolution’-dominated regime, with the Rayleigh number maintained at ${Ra}=10^6$, for (a) ${\varLambda } = 10^2$, and (b) ${\varLambda } = 10^3$. Solid lines represent numerical results, while the dotted and dash-dotted lines depict the analytical solutions of (4.18) and (4.19), respectively.

Figure 11

Figure 12. Characteristics of the interface height during melting. (a) Averaged interface height at ${Ra}=10^6$. (b) Roughness of the interface height at ${Ra}=10^6$, $10^7$ and $10^8$. The colours of the lines correspond to different values of ${\varLambda }$ and are consistent with those described in figure 9. In (a), the black solid line represents the theoretical predictions from (4.22) for the convection regime, the black dashed line from (4.22) for the ‘melting’-dominated diffusion regime, and the black dotted line from (4.25) for the diffusion-dominated regime. The inset in (a) presents the numerical solution for the time evolution of the average height $\bar {h}$ over an extended period for ${\varLambda } = 10^3$, illustrating the very slow dissolution process, which aligns well with the prediction from (4.25) for the diffusion-dominated regime.

Figure 12

Figure 13. Validation test comparing the numerical results of the thermal Nusselt number ${Nu}_T\sim {Ra}_e$ with those provided by Favier et al. (2019), yielding excellent agreement. The dimensionless parameters match those of (Favier et al.2019), with ${St}=0.1$, ${Pr}=1$ and ${Ra}=10^8$.

Figure 13

Figure 14. Grid independence study evaluating the spatial resolution employed in the present investigation. (a) Evolution of the average interface height $\bar {h}(t)$ over time. (b) Visualization of the local reconstructed interface of $x\in [1.5:2.5]$ at $t=5\times 10^{-3}$ using different spatial resolutions from $256\times 64$ to $4096\times 1024$. The simulations are conducted with ${Ra}=10^7$, ${\varLambda } = 1$, while maintaining consistency with all other physical parameters outlined in § 2.

Figure 14

Figure 15. Characteristics of the layering regime transitioning to the convection regime during a long-duration simulation at $({Ra}, {\varLambda }) = (10^7, 2.75)$. (a) Snapshots of the temperature field (left-hand images), solute concentration field (right-hand images) and solid–liquid interfaces (depicted as white solid lines) at various times: $t = 0.1$, $0.5$, $1$, $1.5$, $1.69$, $2$ and $2.6$ (from bottom to top). The colour scheme is consistent with that used in figure 3. (b) The time evolution of the averaged local density ratio $\widetilde {{\varLambda }^*}(z, t)$ along the height in the $(t,z)$ plot. The blue solid line marks the position of the averaged solid–liquid interface.