Hostname: page-component-76d6cb85b7-8p85h Total loading time: 0 Render date: 2026-07-25T09:50:59.045Z Has data issue: false hasContentIssue false

Bendocapillary instability of liquid in a flexible-walled channel

Published online by Cambridge University Press:  16 January 2023

Alexander T. Bradley*
Affiliation:
Mathematical Institute, University of Oxford, Woodstock Rd, Oxford OX2 6GG, UK British Antarctic Survey, High Cross, Madingley Road, Cambridge CB3 0ET, UK
Ian J. Hewitt
Affiliation:
Mathematical Institute, University of Oxford, Woodstock Rd, Oxford OX2 6GG, UK
Dominic Vella
Affiliation:
Mathematical Institute, University of Oxford, Woodstock Rd, Oxford OX2 6GG, UK
*
Email address for correspondence: aleey@bas.ac.uk

Abstract

We study the bendocapillary instability of a liquid droplet that part fills a flexible walled channel. Inspired by experiments in which a periodic pattern emerges as droplets of liquid are condensed slowly into deformable microchannels, we develop a mathematical model of this instability. We describe equilibria of the system, and use a combination of numerical methods and asymptotic analysis in the limit of small channel wall deflections, to elucidate the key features of this instability. We find that configurations are unstable to perturbations of sufficiently small wavenumber regardless of parameter values, that the growth rate of the instability is highly sensitive to the volume of liquid in the channel, and that both wetting and non-wetting configurations are susceptible to the instability in the same channel. Insight into novel interfacial instabilities opens the possibility for their control and thus exploitation in processes such as microfabrication.

Information

Type
JFM Papers
Creative Commons
Creative Common License - CCCreative Common License - BYCreative Common License - SA
This is an Open Access article, distributed under the terms of the Creative Commons Attribution-ShareAlike licence (http://creativecommons.org/licenses/by-sa/4.0), which permits re-use, distribution, and reproduction in any medium, provided the same Creative Commons licence is used to distribute the re-used or adapted article and the original article is properly cited.
Copyright
© The Author(s), 2023. Published by Cambridge University Press.
Figure 0

Figure 1. (a) Snapshots of experiments performed by R. Seemann (personal communication), similar to those published by Seemann et al. (2011), in which liquid droplets are condensed within an array of deformable microchannels. The interaction between the droplets and deformable boundaries leads to a pattern of drops in neighbouring channels offset relative to one another, and with a characteristic droplet spacing and size. (b) Schematic diagram of the experiments shown in panel (a). Here, droplets are shaded blue, flexible channel walls are shaded grey and the base of the array is shaded red. It is not clear in the experiments whether the droplets extend to the base of the channels or not (personal communication). Black dashed lines indicate where the top of the channel walls would be located, if they were undeformed. We refer to variations in the direction parallel to the channel walls as ‘in-plane’ and those perpendicular to that direction as ‘transverse’, as indicated.

Figure 1

Figure 2. Schematic representation of the air–liquid interface in the bendocapillary instability for (a) non-wetting and (b) wetting liquids. In each case, the grey and black outlines indicate the configuration (channel shape and contact line) prior and post perturbation, respectively. Upon perturbing, the contact line is deformed from a straight line to a periodic curve; in both wetting and non-wetting cases, the channel experiences a deformation that enhances (reduces, respectively) the deformation of the channel walls in the base state in regions adjacent to protrusions (invaginations). Note that the configurations shown in this figure are oriented in a way that is rotated $90^{\circ }$ relative to the configuration shown in figure 1(b).

Figure 2

Figure 3. Schematic diagrams of a section of a flexible channel consisting of a solid base and two flexible walls, which are only permitted to bend in the transverse direction. A cut along the centre of the channel (black dashed line) allows the two halves to bend independently of one another. (a) The system is in equilibrium with the meniscus located a distance $x_m$ from the base (the left-hand end, in this orientation). (b) The equilibrium is perturbed by moving the menisci on either side of the cut a distance $\delta$; as described in the main text, if $\lambda$ is sufficiently large, this perturbation results in the flow of liquid from troughs (blue) to peaks (red) with speed $U > 0$, amplifying the perturbation. Note that the configurations shown in this figure are oriented in a direction rotated $90^{\circ }$ relative to the configuration shown in figure 1(b).

Figure 3

Figure 4. (a) Schematic diagram of liquid in a channel consisting of a solid, impenetrable base at $x =0$ and two flexible walls, whose mid-planes are located at $z = \pm h(x,y,t)$. The liquid (a wetting liquid in this case) makes contact with the channel walls at the contact line $x = x_m(y,t)$. The cell extends infinitely in the $y$-direction, only a section of which is shown. (The channel is assumed narrow, $H / L \ll 1$, but here we exaggerate $H/L$ for clarity.) (b) Cross-sections of the system shown in panel (a) through the $(x,y)$ plane (upper) and $(x,z)$ plane (lower); the latter is taken through $y = y^*$, indicated by the dashed box in panel (a).

Figure 4

Figure 5. (a,b) Channel width at the free end, $h_e(x = 1)$, in steady solutions of the model equations (3.19)–(3.29) with (a) $\varGamma = 5$ and (b) $\varGamma = -5$. Where appropriate, the equilibria corresponding to the ‘$+$’ and ‘$-$’ roots in (4.5) are indicated by red and blue curves, respectively (the latter do not exist in the non-wetting case). (c,d) Growth rate $\sigma _u$ of uniform perturbations (i.e. of the form (4.6ac)) to the equilibria corresponding to those shown in panels (a,b), respectively. Each equilibrium is associated with two values of $\sigma _u$, one of which is always zero. (The red and blue $\sigma _u = 0$ curves are indistinguishable for $0.55 \lesssim V \lesssim 0.67$.) The inset in panel (c) is a close up of the section of the main figure indicated by the black dashed box.

Figure 5

Figure 6. (a,b) Growth rates, $\sigma$, and (c) channel width perturbations, $\varLambda(x_0)$, obtained by numerically solving the boundary value problem (5.4)–(5.11) for periodic perturbations with wavenumber $k$ to an equilibrium with cross-sectional volume $V$ (values indicated by the legend). All data correspond to solutions with either $\varGamma = 5$, $a = 0.01$ (solid lines) or $\varGamma = -5$, $a = -0.01$ (dashed lines). Grey-scale lines in panel (c) show the reflection of the $\varGamma = 5$ curves in the line $\boldsymbol{\varLambda}(x_0) = 0$, with darker hues corresponding to larger $V$. The plot in panel (b) is as in panel (a), but zoomed in on the dashed box in panel (a), plotted on logarithmic axes. Note that the solid and dashed lines are almost indistinguishable in panel (b).

Figure 6

Figure 7. Numerically obtained dispersion relations $\sigma (k)$ for cross-sectional volumes (a) $V = 0.1$, (b) $V = 0.2$ and (c) $V = 0.3$ with $a = 0.01$ in each case. In each of panels (ac), the second row is as in the first, but zoomed in around the origin. Within each of panels (ac), each curve corresponds to a different value of $\varGamma$, taking logarithmically spaced values between $10^{-2}$ and $10^{2}$ as indicated by the colourbar on the left-hand side. Here we show only wetting configurations ($\varGamma >0$, $a >0$), but non-wetting configurations behave similarly (see figure 6). (df) Dispersion relations shown in panels (ac), respectively, rescaled according to (5.12a,b).

Figure 7

Figure 8. (a) Numerically obtained values for the normalized perturbation to the channel width $\varLambda(x = x_0)$ and (b) normalized growth rate $\sigma$ as a function of the reduced wavenumber $k/k_c$. Each curve corresponds to a unique $(V,\varGamma )$ pair (the aspect ratio $a = 0.01$ is fixed), whose combination $\epsilon = \varGamma V^4$ is indicated by the colours in the colourbar. The black dashed curves in panels (a,b) correspond to the asymptotic results (6.22) and (6.25a,b), respectively. The numerical results are indistinguishable from the asymptotic curves for $\epsilon \lesssim 10^{-2}$. The inset in panel (b) is a semi-logarithmic plot of the numerically obtained values of the maximum growth rate $\sigma ^*$, rescaled according to (6.25a,b), for $V = 0.1$ (blue), $0.2$ (pink), $0.3$ (green) and $0.4$ (red). (These curves are almost indistinguishable and terminate where the corresponding equilibria cease to exist, having violated the no contact condition (4.4).) The black dashed curve indicates the small-deformation prediction $\sigma ^* = 48\sigma ^*_{SD}$ (6.25a,b).

Figure 8

Figure 9. Difference between successive numerically obtained solutions of the BVP (B1) as a function of $N$, the number of grid points used in the numerical mesh. We show data for three different values of $V$, as indicated in the legend. All results presented here use $a = 0.01$ and $\varGamma = 5$.