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A radiation two-phase flow model for simulating plasma–liquid interactions

Published online by Cambridge University Press:  14 July 2026

Ke-Jian Qian
Affiliation:
State Key Laboratory of High Temperature Gas Dynamics, School of Engineering Science, University of Science and Technology of China , Hefei 230026, PR China
Zhu-Jun Li
Affiliation:
State Key Laboratory of High Temperature Gas Dynamics, School of Engineering Science, University of Science and Technology of China , Hefei 230026, PR China
Tao Tao
Affiliation:
Department of Plasma Physics and Fusion Engineering, University of Science and Technology of China, Hefei 230026, PR China
De-Hua Zhang
Affiliation:
State Key Laboratory of High Temperature Gas Dynamics, School of Engineering Science, University of Science and Technology of China , Hefei 230026, PR China
Rui Yan*
Affiliation:
State Key Laboratory of High Temperature Gas Dynamics, School of Engineering Science, University of Science and Technology of China , Hefei 230026, PR China
Hang Ding*
Affiliation:
State Key Laboratory of High Temperature Gas Dynamics, School of Engineering Science, University of Science and Technology of China , Hefei 230026, PR China
*
Corresponding authors: Rui Yan, ruiyan@ustc.edu.cn; Hang Ding, hding@ustc.edu.cn
Corresponding authors: Rui Yan, ruiyan@ustc.edu.cn; Hang Ding, hding@ustc.edu.cn

Abstract

Content of image described in text.

In laser-produced plasma (LPP) extreme ultraviolet (EUV) sources, deformation of a tin droplet into an optimal target shape is determined by its interaction with a pre-pulse laser-generated plasma. This interaction is mediated by a transient ablation pressure, whose complex spatio-temporal evolution remains experimentally inaccessible. Existing modelling approaches are limited: empirical pressure–impulse models neglect dynamic plasma feedback, while advanced radiation hydrodynamics codes often fail to resolve late-time droplet hydrodynamics. To bridge this gap, we propose a radiation two-phase flow model based on a diffuse interface approach. The model integrates radiation hydrodynamics for the plasma with the Euler equations for a weakly compressible liquid, extending a five-equation diffuse interface formulation to incorporate radiation transport, thermal conduction, ionisation and surface tension. This formulation enforces pressure and velocity equilibrium across the diffuse interface region, with closure models constructed to ensure correct jump conditions at interfaces and asymptotically recover the pure-phase equations in bulk regions. Then we apply the model to simulate a benchmark pre-pulse scenario, where a $50\ \unicode{x03BC} \mathrm{m}$ tin droplet is irradiated by a $10\ \mathrm{ns}$ laser pulse. Our axisymmetric simulations capture the rapid plasma expansion and subsequent inertial flattening of the droplet into a thin, curved sheet over microsecond time scales. Notably, the model reproduces experimentally observed features such as an axial jet – rarely replicated in prior simulations. Quantitative agreement with experimental data for sheet dimensions and velocity validates the approach. The proposed model self-consistently couples laser–plasma physics with compressible droplet dynamics, providing a powerful tool for studying plasma–liquid interactions in LPP-EUV source optimisation.

Information

Type
JFM Papers
Copyright
© The Author(s), 2026. Published by Cambridge University Press
Figure 0

Table 1. The SG parameters for two liquids considered in the present work.Table 1 long description.

Figure 1

Figure 1. (a$a$) Schematic of an interface separating the immiscible plasma and liquid, where the blue phase represents the liquid, and the white phase represents the plasma. (b$b$) A diffuse interface is used to replace the physical interface on a Cartesian grid, and the volume fraction of the liquid αl$\alpha _{l}$ is adopted to represent the interface position, where 0⩽αl⩽1$0\leqslant \alpha _{l}\leqslant 1$.

Figure 2

Figure 2. The profiles of a radiative shock problem at 0 ns$0\ \mathrm{ns}$ (black solid lines and open squares) and 4.2 ns$4.2\ \mathrm{ns}$ (red dashed lines and solid circles), in terms of (a) density, (b) plasma temperature, and (c) radiation temperature. The symbols and lines denote numerical and semi-analytical solutions, respectively. Note that the symbols are sampled at every 8$8$th grid point for visual clarity.

Figure 3

Figure 3. (a) Density, (b) relative density error |ρN−ρA|/ρA$|\rho ^{N}-\rho ^{A}|/\rho ^{A}$, (c) temperature, and (d) relative temperature error |TN−TA|/TA$|T^{N}-T^{A}|/T^{A}$ for the Reinicke–Meyer-ter-Vehn blast wave problem at 0.52 ns$0.52\ \mathrm{ns}$, where superscripts N$N$ and A$A$ represent numerical and semi-analytical results, respectively.

Figure 4

Table 2. Shock-induced bubble collapse compared to prior simulations: collision time (tc$t_{c}$), jet speed at collision (vj$v_{\!j}$), and water-hammer shock pressure (pw$p_{w}$).Table 2 long description.

Figure 5

Figure 4. Numerical results of bubble collapse induced by a planar shock with respect to pressure (upper half) and numerical schlieren (lower half) at (a) 2.2μs$2.2\,\unicode{x03BC} \mathrm{s}$, (b) 3.7μs$3.7\,\unicode{x03BC} \mathrm{s}$, (c) 3.9μs$3.9\,\unicode{x03BC} \mathrm{s}$, (d) 4.1μs$4.1 \,\unicode{x03BC} \mathrm{s}$. The red lines represent the bubble interfaces (by αg=0.5$\alpha _{g} = 0.5$).

Figure 6

Figure 5. Droplet oscillation: (a$a$) evolution of the droplet over an oscillation period, where A$A$ and B$B$ denote the initial semi-axes; (b$b$) kinetic energy of the droplet.

Figure 7

Figure 6. (a$a$) Schematic of axisymmetric simulations of laser–droplet interactions. Cross-sectional shadowgraphs of the droplet at times ranging from t=0.1 μs$t=0.1\ \unicode{x03BC} \mathrm{s}$ to t=1.6 μs$t=1.6\ \unicode{x03BC} \mathrm{s}$: (b$b$g$g$) with surface tension, and (h$h$m$m$) without surface tension. All images have the same spatial scale, as shown in (a$a$).

Figure 8

Figure 7. Numerical results of laser-droplet interaction at (a$a$) 2 ns$2\ \mathrm{ns}$ and (b$b$) 10 ns$10\ \mathrm{ns}$, in terms of density (upper half) and temperature (lower half). The arrows denote velocity vectors, and the black lines represent the droplet shape (by αl=0.5$\alpha _{l}=0.5$).

Figure 9

Figure 8. (a$a$) Normalised surface impulse profiles: the simulation results. The inset shows the polar angle θ$\theta$ in the r$r$z$z$ coordinate. (b$b$) Temporal evolution of the pressure exerted on the droplet surface at θ=0$\theta =0$, pa0$p_{a0}$.

Figure 10

Figure 9. Density contours of the tin sheet at (a$a$) 0.4μs$0.4\,\unicode{x03BC} \mathrm{s}$ and (b$b$) 2μs$2\,\unicode{x03BC} \mathrm{s}$. Insets show side-view experimental shadowgraphs (adapted from Kurilovich et al.2016), superimposed on the simulated drop shape (with respect to the contour of ρ=1.2 gcm−3$\rho =1.2\ \mathrm{g\,cm^{-3}}$) representing the side-view projection.

Figure 11

Figure 10. Propulsion velocity U$U$ of tin droplets as a function of total laser-pulse energy impinging on the droplet EOD$E_{\textit{OD}}$. The experimental data are taken from figure 3(a$a$) of Kurilovich et al. (2016).

Figure 12

Figure 11. Radial expansion of tin droplets as functions of time with different laser-pulse energies: EOD=0.86$E_{\textit{OD}} = 0.86$ and 1.72 mJ$1.72\ \mathrm{mJ}$. The experimental data are taken from figure 4(a$a$) of Kurilovich et al. (2016).